Acetic acid formation from methane and carbon dioxide non-thermal plasma reactions towards an effective carbon fixation

While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no...

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Published inNew journal of chemistry Vol. 46; no. 17; pp. 7855 - 7858
Main Authors Nishimura, Naoyuki, Akaogi, Takayuki, Onishi, Kazuhiro, Tojo, Masahiro
Format Journal Article
Published 03.05.2022
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Summary:While direct CH 3 COOH formation from CH 4 and CO 2 in a non-equilibrium condition is an ideal process, a dielectric-barrier discharge plasma reaction in the presence of CO 2 and isotopic CH 4 ( 13 CH 4 ) revealed that the primly produced CH 3 COOH can comprise both CH 4 -derived carbons ( i.e. , no CO 2 -derived carbon), indicating the importance of a particular CO 2 activation control in non-thermal plasma for an effective carbon fixation. A non-thermal plasma reaction with CO 2 and isotopic CH 4 revealed that the primly produced CH 3 COOH could comprise both CH 4 -derived carbons, indicating the importance of a particular CO 2 activation control for an effective carbon fixation.
Bibliography:https://doi.org/10.1039/d2nj00409g
Electronic supplementary information (ESI) available. See DOI
ISSN:1144-0546
1369-9261
DOI:10.1039/d2nj00409g