Low-temperature catalytic decarboxylation of formic and acetic acid over a Ru/TiO2 catalyst: prospects for continuous production of energy-rich gaseous mixturesElectronic supplementary information (ESI) available. See DOI: 10.1039/c5ra08763e
Catalytic decarboxylation is a novel and promising pathway for continuous and efficient conversion of organic wastewaters. Stable conversion of acetic acid to CH 4 and CO 2 mixtures ( T ≥ 225 °C, S p > 80%, 70 h TOS) was demonstrated. Approaches for overcoming catalyst deactivation during product...
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Main Authors | , , , |
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Format | Journal Article |
Language | English |
Published |
19.06.2015
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Online Access | Get full text |
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Summary: | Catalytic decarboxylation is a novel and promising pathway for continuous and efficient conversion of organic wastewaters. Stable conversion of acetic acid to CH
4
and CO
2
mixtures (
T
≥ 225 °C,
S
p
> 80%, 70 h TOS) was demonstrated. Approaches for overcoming catalyst deactivation during production of H
2
-rich gas from formic acid are outlined.
Long-term continuous reactor operation demonstrates energy-efficient CH
3
COOH conversion pathway and provides appropriate strategies for avoiding unwanted side-reactions with HCOOH feed. |
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Bibliography: | 10.1039/c5ra08763e Electronic supplementary information (ESI) available. See DOI |
ISSN: | 2046-2069 |
DOI: | 10.1039/c5ra08763e |