Probing dark exciton navigation through a local strain landscape in a WSe 2 monolayer
In WSe monolayers, strain has been used to control the energy of excitons, induce funneling, and realize single-photon sources. Here, we developed a technique for probing the dynamics of free excitons in nanoscale strain landscapes in such monolayers. A nanosculpted tapered optical fiber is used to...
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Published in | Nature communications Vol. 13; no. 1; p. 232 |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
England
11.01.2022
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Online Access | Get full text |
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Summary: | In WSe
monolayers, strain has been used to control the energy of excitons, induce funneling, and realize single-photon sources. Here, we developed a technique for probing the dynamics of free excitons in nanoscale strain landscapes in such monolayers. A nanosculpted tapered optical fiber is used to simultaneously generate strain and probe the near-field optical response of WSe
monolayers at 5 K. When the monolayer is pushed by the fiber, its lowest energy states shift by as much as 390 meV (>20% of the bandgap of a WSe
monolayer). Polarization and lifetime measurements of these red-shifting peaks indicate they originate from dark excitons. We conclude free dark excitons are funneled to high-strain regions during their long lifetime and are the principal participants in drift and diffusion at cryogenic temperatures. This insight supports proposals on the origin of single-photon sources in WSe
and demonstrates a route towards exciton traps for exciton condensation. |
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ISSN: | 2041-1723 |