Deposition temperature dependence of thermo-spin and magneto-thermoelectric conversion in Co\(_2\)MnGa films on Y\(_3\)Fe\(_5\)O\(_{12}\) and Gd\(_3\)Ga\(_5\)O\(_{12}\)

• Published in: arXiv.org
• Main Authors: Mizuno, Hayato, Modak, Rajkumar, Hirai, Takamasa, Takahagi, Atsushi, Sakuraba, Yuya, Iguchi, Ryo, Uchida, Ken-ichi
• Format: Paper
• Language: English
• Published: Ithaca Cornell University Library, arXiv.org 18.05.2022
• Subjects: Annealing; Cobalt; Conversion; Crystallization; Electrical conduction; Ettingshausen effect; Gadolinium; Heusler alloys; Iron; Magnetic properties; Peltier effects; Substrates; Temperature dependence; Thermoelectricity; Thermography; Thermomagnetic effects; Yttrium-iron garnet
• ISSN: 2331-8422
• DOI: 10.48550/arxiv.2203.10566

We have characterized Co\(_2\)MnGa (CMG) Heusler alloy films grown on Y\(_3\)Fe\(_5\)O\(_{12}\) (YIG) and Gd\(_3\)Ga\(_5\)O\(_{12}\) (GGG) substrates at different deposition temperatures and investigated thermo-spin and magneto-thermoelectric conversion properties by means of a lock-in thermography technique. X-ray diffraction, magnetization, and electrical transport measurements show that the deposition at high substrate temperatures induces the crystallized structures of CMG while the resistivity of the CMG films on YIG (GGG) prepared at and above 500 {\deg}C (550 {\deg}C) becomes too high to measure the thermo-spin and magneto-thermoelectric effects due to large roughness, highlighting the difficulty of fabricating highly ordered continuous CMG films on garnet structures. Our lock-in thermography measurements show that the deposition at high substrate temperatures results in an increase in the current-induced temperature change for CMG/GGG and a decrease in that for CMG/YIG. The former indicates the enhancement of the anomalous Ettingshausen effect in CMG through crystallization. The latter can be explained by the superposition of the anomalous Ettingshausen effect and the spin Peltier effect induced by the positive (negative) charge-to-spin conversion for the amorphous (crystallized) CMG films. These results provide a hint to construct spin-caloritronic devices based on Heusler alloys.