Controlling the angular emission of a single molecule

Summary form only given. A single fluorescent molecule in an isotropic medium acts as a dipole radiator. In a locally heterogeneous environment the angular emission pattern is modified. Recently Novotny (1996) calculated strongly peaked angular emission when the emitter is brought in close proximity...

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Published inQuantum Electronics and Laser Science Conference (QELS 2000). Technical Digest. Postconference Edition. TOPS Vol.40 (IEEE Cat. No.00CH37089) pp. 16 - 17
Main Authors Gersen, H.-J., Garcia-Parajo, M.F., Veerman, J.-A., Kuipers, L.K., van Hulst, N.F.
Format Conference Proceeding
LanguageEnglish
Published IEEE 2000
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Summary:Summary form only given. A single fluorescent molecule in an isotropic medium acts as a dipole radiator. In a locally heterogeneous environment the angular emission pattern is modified. Recently Novotny (1996) calculated strongly peaked angular emission when the emitter is brought in close proximity to a strong dielectric-metal gradient. We believe we present the first direct observation of this prediction; moreover we show that manipulating the field gradient on a nanometric scale can control the emission direction. Single molecules are detected in near-field optical arrangement.
ISBN:1557526087
9781557526083
ISSN:1094-5695