Scanning tunneling microscopy of Bi$_2$Te$_3$ films prepared by pulsed laser deposition: from nanocrystalline structures to van der Waals epitaxy
Bi$_2$Te$_3$ is a material with high efficiency of thermoelectric energy conversion. Recently, it was also recognized as a topological insulator, and is often used as the basis for creation of other types of topological matter. Pulsed laser deposition (PLD) is widely considered as a simple method fo...
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Main Authors | , , , , |
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Format | Journal Article |
Language | English |
Published |
13.03.2022
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Subjects | |
Online Access | Get full text |
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Summary: | Bi$_2$Te$_3$ is a material with high efficiency of thermoelectric energy
conversion. Recently, it was also recognized as a topological insulator, and is
often used as the basis for creation of other types of topological matter.
Pulsed laser deposition (PLD) is widely considered as a simple method for
growing of multicomponent films, but not as a tool for van der Waals epitaxy.
We demonstrate here that the van der Waals epitaxy of Bi$_2$Te$_3$ is indeed
impossible in vacuum PLD, but is possible in the presence of a background gas,
which is confirmed by the results of scanning tunneling microscopy and
spectroscopy studies. Results of {\it ab initio} calculations reproduce
tunneling spectra of the first three terraces of epitaxial films of
Bi$_2$Te$_3$. In addition, an unusual hexagonal superstructure resembling a
charge-density wave is observed in overheated films. |
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DOI: | 10.48550/arxiv.2203.06734 |