Effect of Electrical Pulse Forms on the CO2 Reforming of Methane using Atmospheric Dielectric Barrier Discharge

• Published in: Plasma chemistry and plasma processing Vol. 24; no. 1; pp. 57 - 72
• Main Authors: Song, H K, Lee, H, Choi, J-W, Na, B-K
• Format: Journal Article
• Language: English
• Published: 01.03.2004
• ISSN: 0272-4324
• DOI: 10.1023/B:PCPP.0000004882.33117.42

Methane conversion using an electric discharge has been studied for many years. Recently, many research groups have developed high frequency pulsed plasma reaction for methane conversion to higher hydrocarbons and synthesis gas. CO2 reforming of methane to synthesis gas has also attracted considerable interest as a method of utilization of the greenhouse gases, CO2 and CH4, which occupy most of man-made greenhouse gases. In this study, the influence of pulse form of applied voltage on methane and carbon dioxide conversions and product selectivity has been investigated using a cylindrical type DBD reactor. For this purpose, two kinds of power supply were compared, that is, AC power supply which has a high frequency sinusoidal wave form, and AC pulse power supply which has modified AC pulse wave form. The conversions of methane and carbon dioxide were enhanced using pulsed plasma. The lower pulse width was more profitable economically.