Nonmagnetic Ground State in RuO_{2} Revealed by Muon Spin Rotation
The magnetic ground state of single crystalline RuO_{2} was investigated by the muon spin rotation and relaxation (μSR) experiment. The spin precession signal due to the spontaneous internal magnetic field B_{loc}, which is expected in the magnetically ordered phase, was not observed in the temperat...
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Published in | Physical review letters Vol. 132; no. 16; p. 166702 |
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Main Authors | , , , , , , |
Format | Journal Article |
Language | English |
Published |
United States
19.04.2024
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Online Access | Get more information |
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Summary: | The magnetic ground state of single crystalline RuO_{2} was investigated by the muon spin rotation and relaxation (μSR) experiment. The spin precession signal due to the spontaneous internal magnetic field B_{loc}, which is expected in the magnetically ordered phase, was not observed in the temperature range 5-400 K. Muon sites were evaluated by first-principles calculations using dilute hydrogen simulating muon as pseudohydrogen, and B_{loc} was simulated for the antiferromagnetic structures with a Ru magnetic moment |m_{Ru}|≈0.05μ_{B} suggested from diffraction experiments. As a result, the possibility was ruled out that muons are localized at sites where B_{loc} accidentally cancels. Conversely, assuming that the slow relaxation observed in μSR spectra was part of the precession signal, the upper limit for the magnitude of |m_{Ru}| was estimated to be 4.8(2)×10^{-4}μ_{B}, which is significantly less than 0.05μ_{B}. These results indicate that the antiferromagnetic order, as reported, is unlikely to exist in the bulk crystal. |
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ISSN: | 1079-7114 |
DOI: | 10.1103/PhysRevLett.132.166702 |