Helimagnetic Structure and Heavy-Fermion-Like Behavior in the Vicinity of the Quantum Critical Point in Mn_{3}P

Antiferromagnet Mn_{3}P with Neel temperature T_{N}=30  K is composed of Mn tetrahedrons and zigzag chains formed by three inequivalent Mn sites. Due to the nearly frustrated lattice with many short Mn-Mn bonds, competition of the exchange interactions is expected. We here investigate the magnetic s...

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Bibliographic Details
Published inPhysical review letters Vol. 124; no. 8; p. 087202
Main Authors Kotegawa, Hisashi, Matsuda, Masaaki, Ye, Feng, Tani, Yuki, Uda, Kohei, Kuwata, Yoshiki, Tou, Hideki, Matsuoka, Eiichi, Sugawara, Hitoshi, Sakurai, Takahiro, Ohta, Hitoshi, Harima, Hisatomo, Takeda, Keiki, Hayashi, Junichi, Araki, Shingo, Kobayashi, Tatsuo C
Format Journal Article
LanguageEnglish
Published United States 28.02.2020
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Summary:Antiferromagnet Mn_{3}P with Neel temperature T_{N}=30  K is composed of Mn tetrahedrons and zigzag chains formed by three inequivalent Mn sites. Due to the nearly frustrated lattice with many short Mn-Mn bonds, competition of the exchange interactions is expected. We here investigate the magnetic structure and physical properties including pressure effect in single crystals of this material, and reveal a complex yet well-ordered helimagnetic structure. The itinerant character of this materials is strong, and the ordered state with small magnetic moments is easily suppressed under pressure, exhibiting a quantum critical point at ∼1.6  GPa. The remarkable mass renormalization, even in the ordered state, and an incoherent-coherent crossover in the low-temperature region, characterize an unusual electronic state in Mn_{3}P, which is most likely effected by the underlying frustration effect.
ISSN:1079-7114
DOI:10.1103/PhysRevLett.124.087202