Large phonon thermal Hall conductivity in the antiferromagnetic insulator Cu3TeO6

Phonons are known to generate a thermal Hall effect in certain insulators, including oxides with rare-earth impurities, quantum paraelectrics, multiferroic materials, and cuprate Mott insulators. In each case, a special feature of the material is presumed relevant for the underlying mechanism that c...

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Published inProceedings of the National Academy of Sciences - PNAS Vol. 119; no. 34; p. 1
Main Authors Chen, Lu, Boulanger, Marie-Eve, Wang, Zhi-Cheng, Tafti, Fazel, Taillefer, Louis
Format Journal Article
LanguageEnglish
Published Washington National Academy of Sciences 23.08.2022
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Summary:Phonons are known to generate a thermal Hall effect in certain insulators, including oxides with rare-earth impurities, quantum paraelectrics, multiferroic materials, and cuprate Mott insulators. In each case, a special feature of the material is presumed relevant for the underlying mechanism that confers chirality to phonons in a magnetic field. A fundamental question is whether a phonon Hall effect is an unusual occurrence-linked to special characteristics such as skew scattering off rare-earth impurities, structural domains, ferroelectricity, or ferromagnetism-or a much more common property of insulators than hitherto believed. To help answer this question, we have turned to a material with none of the previously encountered special features: the cubic antiferromagnet Cu3TeO6. We find that its thermal Hall conductivity κxy is among the largest of any insulator so far. We show that this record-high κxy signal is due to phonons, and it does not require the presence of magnetic order, as it persists above the ordering temperature. We conclude that the phonon Hall effect is likely to be a fairly common property of solids.
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1L.C. and M.-E.B. contributed equally to this work.
Edited by J. C. Davis, University of Oxford, United Kingdom; received May 16, 2022; accepted July 18, 2022
Author contributions: L.C., M.-E.B., and L.T. designed research; L.C. and M.-E.B. performed research; L.C. and M.-E.B. analyzed data; L.C., M.-E.B., Z.-C.W., F.T., and L.T. wrote the paper; and Z.-C.W. and F.T. provided the samples.
ISSN:0027-8424
1091-6490
1091-6490
DOI:10.1073/pnas.2208016119