Monolayer MoS2 Films Supported by 3D Nanoporous Metals for High-Efficiency Electrocatalytic Hydrogen Production

The “edge‐free” monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out‐of‐plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bendin...

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Bibliographic Details
Published inAdvanced materials (Weinheim) Vol. 26; no. 47; pp. 8023 - 8028
Main Authors Tan, Yongwen, Liu, Pan, Chen, Luyang, Cong, Weitao, Ito, Yoshikazu, Han, Jiuhui, Guo, Xianwei, Tang, Zheng, Fujita, Takeshi, Hirata, Akihiko, Chen, Mingwei W.
Format Journal Article
LanguageEnglish
Published Germany Blackwell Publishing Ltd 17.12.2014
Subjects
2D materials
hydrogen evolution reaction
molybdenum disulphide
monolayer dichalcogenide
nanoporous metal
nanoporous metal
monolayer dichalcogenide
molybdenum disulphide
2D materials
hydrogen evolution reaction
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Summary:The “edge‐free” monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out‐of‐plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor‐to‐metal transition of 2H MoS2 and the formation of catalytically active sites for HER.
Bibliography:ark:/67375/WNG-BM11VRC2-6
ArticleID:ADMA201403808
istex:EB3D5C6546185D625C6A3B96A5445E43A965C270
ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:0935-9648
1521-4095
1521-4095
DOI:10.1002/adma.201403808