Impact of epitaxial strain relaxation on ferromagnetism in a freestanding La2 / 3Sr1 / 3MnO3 membrane

Manganite perovskites host emerging physical properties of strongly-correlated electrons with charge, spin, and lattice degrees of freedom. Using the epitaxial lift-off technique, we report enhancement of saturation magnetization and the ferromagnetic transition temperature of freestanding La2/3Sr1/...

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Bibliographic Details
Published inJapanese Journal of Applied Physics Vol. 62; no. 10; pp. 100902 - 100906
Main Authors Atsumi, Ryuji, Shiogai, Junichi, Yamazaki, Takumi, Seki, Takeshi, Ueda, Kohei, Matsuno, Jobu
Format Journal Article
LanguageEnglish
Published Tokyo IOP Publishing 01.10.2023
Japanese Journal of Applied Physics
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Summary:Manganite perovskites host emerging physical properties of strongly-correlated electrons with charge, spin, and lattice degrees of freedom. Using the epitaxial lift-off technique, we report enhancement of saturation magnetization and the ferromagnetic transition temperature of freestanding La2/3Sr1/3MnO3 membrane compared with as-grown film on SrTiO3 substrate involving lateral tensile strain. Structural analysis reveals shrinkage of unit-cell volume by tensile strain relaxation in the freestanding membrane, which causes enhancement of the ferromagnetic interaction. The impact of the microscopic lattice deformation on the ferromagnetism of La2/3Sr1/3MnO3 indicates a high potential of this material for flexible electronics applications with intriguing functionalities in strongly-correlated electron systems.
Bibliography:JJAP-105410
ISSN:0021-4922
1347-4065
DOI:10.35848/1347-4065/ad0270