MOF-derived bimetallic core–shell catalyst HZSM-5@ZrO 2 –In 2 O 3 : high CO 2 conversion in reverse water gas shift reaction

The bicomponent core–shell catalyst HZSM-5@ZrO 2 –In 2 O 3 was synthesized via the decomposition of In(NO 3 ) 3 /HZSM-5@UIO-66, which was obtained by impregnating HZSM-5@UIO-66 with In(NO 3 ) 3 solution. The bimetallic oxide particles of ZrO 2 –In 2 O 3 were formed through the simultaneous decomposi...

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Published inMaterials chemistry frontiers Vol. 6; no. 19; pp. 2826 - 2834
Main Authors Fang, Huimin, Zhao, Guofeng, Cheng, Denghui, Liu, Jichang, Lan, Dengpeng, Jiang, Qi, Liu, Xuqiang, Ge, Jianping, Xu, Zhenliang, Xu, Haitao
Format Journal Article
LanguageEnglish
Published 26.09.2022
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Summary:The bicomponent core–shell catalyst HZSM-5@ZrO 2 –In 2 O 3 was synthesized via the decomposition of In(NO 3 ) 3 /HZSM-5@UIO-66, which was obtained by impregnating HZSM-5@UIO-66 with In(NO 3 ) 3 solution. The bimetallic oxide particles of ZrO 2 –In 2 O 3 were formed through the simultaneous decomposition of UIO-66 and In(NO 3 ) 3 , and were anchored to the surface of the HZSM-5 core. The HZSM-5@ZrO 2 –In 2 O 3 catalyst exhibited 31.1% CO 2 conversion with 96.3% CO selectivity at 400 °C for the reverse water gas shift reaction.
ISSN:2052-1537
2052-1537
DOI:10.1039/D2QM00307D