Spin Disorder on a Triangular Lattice

As liquids crystallize into solids on cooling, spins in magnets generally form periodic order. However, three decades ago, it was theoretically proposed that spins on a triangular lattice form a liquidlike disordered state at low temperatures. Whether or not a spin liquid is stabilized by geometrica...

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Published inScience (American Association for the Advancement of Science) Vol. 309; no. 5741; pp. 1697 - 1700
Main Authors Nakatsuji, Satoru, Nambu, Yusuke, Tonomura, Hiroshi, Sakai, Osamu, Jonas, Seth, Broholm, Collin, Tsunetsugu, Hirokazu, Qiu, Yiming, Maeno, Yoshiteru
Format Journal Article
LanguageEnglish
Published Washington, DC American Association for the Advancement of Science 09.09.2005
The American Association for the Advancement of Science
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Summary:As liquids crystallize into solids on cooling, spins in magnets generally form periodic order. However, three decades ago, it was theoretically proposed that spins on a triangular lattice form a liquidlike disordered state at low temperatures. Whether or not a spin liquid is stabilized by geometrical frustration has remained an active point of inquiry ever since. Our thermodynamic and neutron measurements on NiGa₂S₄, a rare example of a two-dimensional triangular lattice antiferromagnet, demonstrate that geometrical frustration stabilizes a low-temperature spin-disordered state with coherence beyond the two-spin correlation length. Spin liquid formation may be an origin of such behavior.
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ISSN:0036-8075
1095-9203
DOI:10.1126/science.1114727