An AIEgen-based 3D covalent organic framework for white light-emitting diodes
The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m 2 g −1 ). According to powder X-ray diffraction and con...
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| Published in | Nature communications Vol. 9; no. 1; pp. 5234 - 7 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
07.12.2018
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m
2
g
−1
). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated
pts
topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future.
3D covalent organic frameworks (COF) show interesting hierarchical arrangements of nanopores and open sites but their synthesis remains challenging. Here the authors report a fluorescent AIEgen-based 3D COF and demonstrate application as a coating material for white LEDs and for sensing of picric acid |
|---|---|
| AbstractList | 3D covalent organic frameworks (COF) show interesting hierarchical arrangements of nanopores and open sites but their synthesis remains challenging. Here the authors report a fluorescent AIEgen-based 3D COF and demonstrate application as a coating material for white LEDs and for sensing of picric acid The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m g ). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m2 g-1). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future.The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m2 g-1). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m2 g−1). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m 2 g −1 ). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m(2)g(-1)). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design and synthesis of an AIEgen-based 3D COF (3D-TPE-COF), with a high surface area (1084 m 2 g −1 ). According to powder X-ray diffraction and continuous rotation electron diffraction analyses, 3D-TPE-COF is identified to adopt a seven-fold interpenetrated pts topology. Interestingly, 3D-TPE-COF emits yellow fluorescence upon excitation, with a photoluminescence quantum yield of 20%. Moreover, by simply coating 3D-TPE-COF onto a commercial blue light-emitting diode (LED), a prototype white LED (WLED) under continuously driving without degradation for 1200 h was demonstrated. The present work suggests the possibility of using COF materials for stable WLEDs, which will greatly inspire us to design and synthesize fluorescent 3D COFs and facilitate the development of COF-based WLEDs in future. 3D covalent organic frameworks (COF) show interesting hierarchical arrangements of nanopores and open sites but their synthesis remains challenging. Here the authors report a fluorescent AIEgen-based 3D COF and demonstrate application as a coating material for white LEDs and for sensing of picric acid |
| ArticleNumber | 5234 |
| Author | Ding, Huimin Chen, Rufan Lin, Guiqing Wang, Cheng Yang, Chuluo Peng, Zhengkang Sun, Junliang Li, Jian Xie, Guohua Wang, Baoshan |
| Author_xml | – sequence: 1 givenname: Huimin surname: Ding fullname: Ding, Huimin organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 2 givenname: Jian surname: Li fullname: Li, Jian organization: College of Chemistry and Molecular Engineering, Beijing National Laboratory for Molecular Sciences, Peking University, Department of Materials and Environmental Chemistry, Stockholm University – sequence: 3 givenname: Guohua orcidid: 0000-0003-0764-7889 surname: Xie fullname: Xie, Guohua organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 4 givenname: Guiqing surname: Lin fullname: Lin, Guiqing organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 5 givenname: Rufan surname: Chen fullname: Chen, Rufan organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 6 givenname: Zhengkang surname: Peng fullname: Peng, Zhengkang organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 7 givenname: Chuluo orcidid: 0000-0001-9337-3460 surname: Yang fullname: Yang, Chuluo organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 8 givenname: Baoshan orcidid: 0000-0003-3417-9283 surname: Wang fullname: Wang, Baoshan organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University – sequence: 9 givenname: Junliang orcidid: 0000-0003-4074-0962 surname: Sun fullname: Sun, Junliang email: junliang.sun@pku.edu.cn organization: College of Chemistry and Molecular Engineering, Beijing National Laboratory for Molecular Sciences, Peking University, Department of Materials and Environmental Chemistry, Stockholm University – sequence: 10 givenname: Cheng surname: Wang fullname: Wang, Cheng email: chengwang@whu.edu.cn organization: Key Laboratory of Biomedical Polymers (Ministry of Education), College of Chemistry and Molecular Sciences, Wuhan University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30532031$$D View this record in MEDLINE/PubMed https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-163700$$DView record from Swedish Publication Index |
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| Snippet | The design and synthesis of three-dimensional covalent organic frameworks (3D COFs) have still been considered as a big challenge. Here we report the design... 3D covalent organic frameworks (COF) show interesting hierarchical arrangements of nanopores and open sites but their synthesis remains challenging. Here the... |
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| SubjectTerms | 147/28 639/638/298/921 639/638/455/941 Design Electron diffraction Fluorescence Humanities and Social Sciences Light emitting diodes multidisciplinary Organic light emitting diodes Photoluminescence Photons Science Science (multidisciplinary) Synthesis Topology White light X ray powder diffraction X-ray diffraction |
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| Title | An AIEgen-based 3D covalent organic framework for white light-emitting diodes |
| URI | https://link.springer.com/article/10.1038/s41467-018-07670-4 https://www.ncbi.nlm.nih.gov/pubmed/30532031 https://www.proquest.com/docview/2151751380 https://www.proquest.com/docview/2155153512 https://pubmed.ncbi.nlm.nih.gov/PMC6286360 https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-163700 https://doaj.org/article/88a34ab66c5747ffaae9c73f11c7120e |
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