Dynamic self-assembly of magnetized, millimetre-sized objects rotating at a liquid–air interface

• Published in: Nature (London) Vol. 405; no. 6790; pp. 1033 - 1036
• Main Authors: Grzybowski, Bartosz A., Stone, Howard A., Whitesides, George M.
• Format: Journal Article
• Language: English
• Published: London Nature Publishing Group UK 29.06.2000; Nature Publishing; Nature Publishing Group
• Subjects: Chemistry; Dynamical systems; Dynamics; Exact sciences and technology; Fluid dynamics; Fluid flow; Fundamental areas of phenomenology (including applications); Humanities and Social Sciences; letter; Magnetic fields; Magnetism; multidisciplinary; Multiphase and particle-laden flows; Nonhomogeneous flows; Order disorder; Physics; Rotating; Science; Self assembly; Vortices; Gas liquid interface; Self assembly; Patterning; Self organization; Rotating disk; Particle suspension; Magnetic fields; Experimental study
• ISSN: 0028-0836; 1476-4687; 1476-4687
• DOI: 10.1038/35016528

Spontaneous pattern formation by self-assembly is of long-standing 1 , 2 , 3 and continuing interest 4 , 5 not only for its aesthetic appeal 6 , 7 , but also for its fundamental 8 , 9 , 10 , 11 , 12 , 13 , 14 , 15 , 16 , 17 , 18 and technological relevance 19 . So far, the study of self-organization processes has mainly focused on static structures, but dynamic systems 20 , 21 , 22 —those that develop order only when dissipating energy—are of particular interest for studying complex behaviour 23 , 24 . Here we describe the formation of dynamic patterns of millimetre-sized magnetic disks at a liquid–air interface, subject to a magnetic field produced by a rotating permanent magnet. The disks spin around their axes with angular frequency equal to that of the magnet, and are attracted towards its axis of rotation while repelling each other. This repulsive hydrodynamic interaction is due to fluid motion associated with spinning; the interplay between attractive and repulsive interactions leads to the formation of patterns exhibiting various types of ordering, some of which are entirely new. This versatile system should lead to a better understanding of dynamic self-assembly, while providing a test-bed for stability theories of interacting point vortices 25 , 26 , 27 , 28 and vortex patches 29 .