Fabrication of a Au/Si nanocomposite structure by nanosecond pulsed laser irradiation

A gold/silicon nanocomposite structure (NCS) was formed on a Si(100) surface by nanosecond pulsed laser irradiation. The Au/Si NCS contained both Au nanoparticles (NPs) and Au-Si alloy layers. We report that the use of laser irradiation to form Au NPs comprises two competing processes: a top-down ef...

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Published inNanotechnology Vol. 22; no. 37; pp. 375607 - 1-7
Main Authors Yoshida, Yutaka, Watanabe, Seiichi, Nishijima, Yoshiaki, Ueno, Kosei, Misawa, Hiroaki, Kato, Takahiko
Format Journal Article
LanguageEnglish
Published England IOP Publishing 16.09.2011
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Summary:A gold/silicon nanocomposite structure (NCS) was formed on a Si(100) surface by nanosecond pulsed laser irradiation. The Au/Si NCS contained both Au nanoparticles (NPs) and Au-Si alloy layers. We report that the use of laser irradiation to form Au NPs comprises two competing processes: a top-down effect involving decomposition into smaller NPs and a bottom-up effect involving self-assembly or self-organization into larger NPs. The formation of the periodic structure involved self-organization, i.e., the bottom-up effect, and was observed in situ using a pulsed-laser-equipped high-voltage electron microscope. The NCS formed by laser irradiation can be controlled by adjusting the laser energy density and the number of laser pulses.
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ISSN:0957-4484
1361-6528
DOI:10.1088/0957-4484/22/37/375607