Deterministic control of ferroelectric polarization by ultrafast laser pulses

Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a h...

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Published inNature communications Vol. 13; no. 1; p. 2566
Main Authors Chen, Peng, Paillard, Charles, Zhao, Hong Jian, Íñiguez, Jorge, Bellaiche, Laurent
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 10.05.2022
Nature Publishing Group
Nature Portfolio
Subjects
119/118
639/301/1005/1007
639/624/400/561
639/766/119/996
639/766/400/561
Anharmonicity
Electric polarization
Ferroelectric materials
Ferroelectricity
Humanities and Social Sciences
Light effects
multidisciplinary
Phase transitions
Phonons
Physics
Polarization
Room temperature
Science
Science (multidisciplinary)
Stimuli
Ultrafast lasers
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Abstract Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices. Controlling the electric polarization in ferroelectric materials at room temperature is an important aspect in the design of novel ferroelectric-based devices. Simulations of a typical ferroelectric material now provide insights into why and how its ferroelectric polarization can be partially reversed.
AbstractList Abstract Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices.
Abstract Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices.
Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices. Controlling the electric polarization in ferroelectric materials at room temperature is an important aspect in the design of novel ferroelectric-based devices. Simulations of a typical ferroelectric material now provide insights into why and how its ferroelectric polarization can be partially reversed.
Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices.Controlling the electric polarization in ferroelectric materials at room temperature is an important aspect in the design of novel ferroelectric-based devices. Simulations of a typical ferroelectric material now provide insights into why and how its ferroelectric polarization can be partially reversed.
Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for designing novel ferroelectric-based devices. One emergent light-induced technique for controlling polarization consists in anharmonically driving a high-frequency phonon mode through its coupling to the polarization. A step towards such control has been recently accomplished, but the polarization has been reported to be only partially reversed and for a short lapse of time. Such transient partial reversal is not currently understood, and it is presently unclear if full control of polarization, by, e.g., fully reversing it or even making it adopt different directions (thus inducing structural phase transitions), can be achieved by activating the high-frequency phonon mode via terahertz pulse stimuli. Here, by means of realistic simulations of a prototypical ferroelectric, we reveal and explain (1) why a transient partial reversal has been observed, and (2) how to deterministically control the ferroelectric polarization thanks to these stimuli. Such results can provide guidance for realizing original ultrafast optoferroic devices.
Controlling the electric polarization in ferroelectric materials at room temperature is an important aspect in the design of novel ferroelectric-based devices. Simulations of a typical ferroelectric material now provide insights into why and how its ferroelectric polarization can be partially reversed.
ArticleNumber 2566
Author Zhao, Hong Jian
Paillard, Charles
Bellaiche, Laurent
Chen, Peng
Íñiguez, Jorge
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  givenname: Hong Jian
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  organization: Physics Department and Institute for Nanoscience and Engineering, University of Arkansas, International Center for Computational Method and Software (ICCMS) and Key Laboratory of Physics and Technology for Advanced Batteries, Jilin University
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  surname: Bellaiche
  fullname: Bellaiche, Laurent
  email: laurent@uark.edu
  organization: Physics Department and Institute for Nanoscience and Engineering, University of Arkansas
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Snippet Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for...
Abstract Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for...
Abstract Ultrafast light-matter interactions present a promising route to control ferroelectric polarization at room temperature, which is an exciting idea for...
Controlling the electric polarization in ferroelectric materials at room temperature is an important aspect in the design of novel ferroelectric-based devices....
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StartPage 2566
SubjectTerms 119/118
639/301/1005/1007
639/624/400/561
639/766/119/996
639/766/400/561
Anharmonicity
Electric polarization
Ferroelectric materials
Ferroelectricity
Humanities and Social Sciences
Light effects
multidisciplinary
Phase transitions
Phonons
Physics
Polarization
Room temperature
Science
Science (multidisciplinary)
Stimuli
Ultrafast lasers
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Title Deterministic control of ferroelectric polarization by ultrafast laser pulses
URI https://link.springer.com/article/10.1038/s41467-022-30324-5
https://www.ncbi.nlm.nih.gov/pubmed/35538101
https://www.proquest.com/docview/2661733549
https://search.proquest.com/docview/2662541231
https://centralesupelec.hal.science/hal-03664634
https://pubmed.ncbi.nlm.nih.gov/PMC9090784
https://doaj.org/article/5c91e196ff864b0fbc2c60a072b7579c
Volume 13
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