Relative importance of high-latitude local and long-range-transported dust for Arctic ice-nucleating particles and impacts on Arctic mixed-phase clouds

• Published in: Atmospheric chemistry and physics Vol. 22; no. 4; pp. 2909 - 2935
• Main Authors: Shi, Yang, Liu, Xiaohong, Wu, Mingxuan, Zhao, Xi, Ke, Ziming, Brown, Hunter
• Format: Journal Article
• Language: English
• Published: Katlenburg-Lindau Copernicus GmbH 03.03.2022; Copernicus Publications, EGU; Copernicus Publications
• Subjects: Aerosols; Arctic clouds; Arctic ice; Atmosphere; Atmospheric particulates; Boundary layers; Cloud properties; Clouds; Comparative analysis; Cooling; Cooling effects; Downwelling; Dust; Dust particles; Dust storms; Emissions; Energy budget; ENVIRONMENTAL SCIENCES; Experiments; Force and energy; Latitude; Long-range transport; Lower troposphere; Marking and tracking techniques; Polar environments; Regional climates; Surface energy; Surface properties; Troposphere; Upper troposphere; Vertical advection; Arctic; Arctic region; Greenland
• ISSN: 1680-7324; 1680-7316; 1680-7324
• DOI: 10.5194/acp-22-2909-2022

Dust particles, serving as ice-nucleating particles (INPs), may impact the Arctic surface energy budget and regional climate by modulating the mixed-phase cloud properties and lifetime. In addition to long-range transport from low-latitude deserts, dust particles in the Arctic can originate from local sources. However, the importance of high-latitude dust (HLD) as a source of Arctic INPs (compared to low-latitude dust, LLD) and its effects on Arctic mixed-phase clouds are overlooked. In this study, we evaluate the contribution to Arctic dust loading and INP population from HLD and six LLD source regions by implementing a source-tagging technique for dust aerosols in version 1 of the US Department of Energy's Energy Exascale Earth System Model (E3SMv1). Our results show that HLD is responsible for 30.7 % of the total dust burden in the Arctic, whereas LLD from Asia and North Africa contributes 44.2 % and 24.2 %, respectively. Due to its limited vertical transport as a result of stable boundary layers, HLD contributes more in the lower troposphere, especially in boreal summer and autumn when the HLD emissions are stronger. LLD from North Africa and East Asia dominates the dust loading in the upper troposphere with peak contributions in boreal spring and winter. The modeled INP concentrations show better agreement with both ground and aircraft INP measurements in the Arctic when including HLD INPs. The HLD INPs are found to induce a net cooling effect (−0.24 W m−2 above 60∘ N) on the Arctic surface downwelling radiative flux by changing the cloud phase of the Arctic mixed-phase clouds. The magnitude of this cooling is larger than that induced by North African and East Asian dust (0.08 and −0.06 W m−2, respectively), mainly due to different seasonalities of HLD and LLD. Uncertainties of this study are discussed, which highlights the importance of further constraining the HLD emissions.