Spectroscopy of a tunable moiré system with a correlated and topological flat band

Moiré superlattices created by the twisted stacking of two-dimensional crystals can host electronic bands with flat energy dispersion in which enhanced interactions promote correlated electron states. The twisted double bilayer graphene (TDBG), where two Bernal bilayer graphene are stacked with a tw...

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Published inNature communications Vol. 12; no. 1; pp. 2732 - 7
Main Authors Liu, Xiaomeng, Chiu, Cheng-Li, Lee, Jong Yeon, Farahi, Gelareh, Watanabe, Kenji, Taniguchi, Takashi, Vishwanath, Ashvin, Yazdani, Ali
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 12.05.2021
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Summary:Moiré superlattices created by the twisted stacking of two-dimensional crystals can host electronic bands with flat energy dispersion in which enhanced interactions promote correlated electron states. The twisted double bilayer graphene (TDBG), where two Bernal bilayer graphene are stacked with a twist angle, is such a moiré system with tunable flat bands. Here, we use gate-tuned scanning tunneling spectroscopy to directly demonstrate the tunability of the band structure of TDBG with an electric field and to show spectroscopic signatures of electronic correlations and topology for its flat band. Our spectroscopic experiments are in agreement with a continuum model of TDBG band structure and reveal signatures of a correlated insulator gap at partial filling of its isolated flat band. The topological properties of this flat band are probed with the application of a magnetic field, which leads to valley polarization and the splitting of Chern bands with a large effective g-factor. Twisted double bilayer graphene hosts flat bands that can be tuned with an electric field. Here, by using gate-tuned scanning tunneling spectroscopy, the authors demonstrate the tunability of the flat band and reveal spectral signatures of correlated electron states and the topological nature of the flat band.
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MEXT
CREST
JSPS KAKENHI
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Gordon and Betty Moore Foundation
National Science Foundation (NSF)
FG02-07ER46419; GBMF4530; GBMF9469; DMR-1420541; DMR-1904442; DMR-2011750; JPMXP0112101001; JP20H00354; JPMJCR15F3
ISSN:2041-1723
2041-1723
DOI:10.1038/s41467-021-23031-0