Thermal conductivity measurements via time-domain thermoreflectance for the characterization of radiation induced damage
The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation dama...
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| Published in | Journal of materials research Vol. 30; no. 9; pp. 1403 - 1412 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
New York, USA
Cambridge University Press
14.05.2015
Springer International Publishing Springer Nature B.V Materials Research Society |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 ± 1.8 W m−1 K−1 at room temperature. Furthermore, we find that the thermal conductivities of copper–niobium nanostructured multilayers do not change with helium ion irradiation doses of 1015 cm−2 and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. |
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| AbstractList | Abstract
The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 ± 1.8 W m
−1
K
−1
at room temperature. Furthermore, we find that the thermal conductivities of copper–niobium nanostructured multilayers do not change with helium ion irradiation doses of 10
15
cm
−2
and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 ± 1.8 W m-1 K-1 at room temperature. Furthermore, we find that the thermal conductivities of copper-niobium nanostructured multilayers do not change with helium ion irradiation doses of 1015 cm-2 and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 ± 1.8 W m −1 K −1 at room temperature. Furthermore, we find that the thermal conductivities of copper–niobium nanostructured multilayers do not change with helium ion irradiation doses of 10 15 cm −2 and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. The progressive build up of displacement damage and fission products inside different systems and components of a nuclear reactor can lead to significant defect formation, degradation, and damage of the constituent materials. This structural modification can highly influence the thermal transport mechanisms and various mechanical properties of solids. In this paper we demonstrate the use of time-domain thermoreflectance (TDTR), a non-destructive method capable of measuring the thermal transport in material systems from nano to bulk scales, to study the effect of radiation damage and the subsequent changes in the thermal properties of materials. We use TDTR to show that displacement damage from ion irradiation can significantly reduce the thermal conductivity of Optimized ZIRLO, a material used as fuel cladding in several current nuclear reactors. We find that the thermal conductivity of copper-niobium nanostructured multilayers does not change with helium ion irradiation doses of up to 1015 cm-2 and ion energy of 200 keV suggesting that these structures can be used and radiation tolerant materials in nuclear reactors. We compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Results demonstrate that TDTR thermal measurements can be used to quantify depth dependent damage. The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 - 1.8 W m1 K1 at room temperature. Furthermore, we find that the thermal conductivities of copperniobium nanostructured multilayers do not change with helium ion irradiation doses of 1015 cm2 and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We demonstrate the use of time-domain thermoreflectance (TDTR), a nondestructive thermal measurement technique, to study the effects of radiation damage on material properties. We use TDTR to report on the thermal conductivity of optimized ZIRLO, a material used as fuel cladding in nuclear reactors. We find that the thermal conductivity of optimized ZIRLO is 10.7 ± 1.8 W m−1 K−1 at room temperature. Furthermore, we find that the thermal conductivities of copper–niobium nanostructured multilayers do not change with helium ion irradiation doses of 1015 cm−2 and ion energy of 200 keV, demonstrating the potential of heterogeneous multilayer materials for radiation tolerant coatings. Finally, we compare the effect of ion doses and ion beam energies on the measured thermal conductivity of bulk silicon. Our results demonstrate that TDTR can be used to quantify depth dependent damage. |
| Author | Hattar, Khalid Misra, Amit Cheaito, Ramez Hopkins, Patrick E. Gorham, Caroline S. |
| Author_xml | – sequence: 1 givenname: Ramez surname: Cheaito fullname: Cheaito, Ramez organization: Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904, USA – sequence: 2 givenname: Caroline S. surname: Gorham fullname: Gorham, Caroline S. organization: Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904, USA – sequence: 3 givenname: Amit surname: Misra fullname: Misra, Amit organization: † Department of Material Science and Engineering, University of Michigan, Ann Arbor, Michigan 48109, USA – sequence: 4 givenname: Khalid surname: Hattar fullname: Hattar, Khalid email: khattar@sandia.gov organization: ‡ Sandia National Laboratories, Albuquerque, New Mexico 87185, USA – sequence: 5 givenname: Patrick E. surname: Hopkins fullname: Hopkins, Patrick E. email: phopkins@virginia.edu organization: § Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904, USA |
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| Snippet | The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials. We... Abstract The progressive build up of fission products inside different nuclear reactor components can lead to significant damage of the constituent materials.... The progressive build up of displacement damage and fission products inside different systems and components of a nuclear reactor can lead to significant... |
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| SubjectTerms | Accumulation Analysis Applied and Technical Physics Biomaterials Conductivity Damage Editors Electron microscopes Energy (nuclear) GENERAL STUDIES OF NUCLEAR REACTORS Heat conductivity Heat transfer Inorganic Chemistry Lasers Materials Engineering Materials research MATERIALS SCIENCE Measurement techniques Microscopy Multilayers Nanostructure Nanostructured materials Nanotechnology Nuclear fission Nuclear fuels Nuclear reactor components Nuclear reactors Point defects Radiation Silicon Studies Thermal conductivity Thermal measurements |
| Title | Thermal conductivity measurements via time-domain thermoreflectance for the characterization of radiation induced damage |
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