SdH Oscillations from the Dirac Surface State in the Fermi‐Arc Antiferromagnet NdBi

• Published in: Advanced science Vol. 10; no. 35; pp. e2303978 - n/a
• Main Authors: Wang, Ruoqi, Zhang, Junchao, Li, Tian, Chen, Keming, Li, Zhengyu, Wu, Mingliang, Ling, Langsheng, Xi, Chuanying, Hong, Kunquan, Miao, Lin, Yuan, Shijun, Chen, Taishi, Wang, Jinlan
• Format: Journal Article
• Language: English
• Published: Germany John Wiley & Sons, Inc 01.12.2023; John Wiley and Sons Inc; Wiley
• Subjects: AFM spintronics; Crystal structure; Electrons; Fermi‐arc; Magnetic fields; NdBi; orbital magnetic moment; peculiar surface state; spin‐flop transition; Symmetry; Temperature; NdBi; Fermi-arc; peculiar surface state; AFM spintronics; orbital magnetic moment; spin-flop transition
• ISSN: 2198-3844; 2198-3844
• DOI: 10.1002/advs.202303978

The recent progress in CuMnAs and Mn3X (X = Sn, Ge, Pt) shows that antiferromagnets (AFMs) provide a promising platform for advanced spintronics device innovations. Most recently, a switchable Fermi‐arc is discovered by the ARPES technique in antiferromagnet NdBi, but the knowledge about electron‐transport property and the manipulability of the magnetic structure in NdBi is still vacant to date. In this study, SdH oscillations are successfully verified from the Dirac surface states (SSs) with 2‐dimensionality and nonzero Berry phase. Particularly, it is observed that the spin‐flop transition only appears when the external magnetical field is applied along [001] direction, and features obvious hysteresis for the first time in NdBi, which provides a powerful handle for adjusting the spin texture in NdBi. Crucially, the DFT shows the Dirac cone and the Fermi arc strongly depend on the high‐order magnetic structure of NdBi and further reveals the orbital magnetic moment of Nd plays a crucial role in fostering the peculiar SSs, leading to unveil the mystery of the band‐splitting effect and to manipulate the electronic transport, high‐effectively, in the thin film works in NdBi. It is believed that this study provides important guidance for the development of new antiferromagnet‐based spintronics devices based on cutting‐edge rare‐earth monopnictides. In Fermi‐arc antiferromagnet NdBi, it is first achieved 1) the SdH oscillations from the Dirac surface state with 2‐dimensionality and nonzero Berry, 2) the manipulation of the magnetic structure by spin‐flop transition with obvious hysteresis, 3) DFT revealing the peculiar surface states strongly depending on the high‐order magnetic structure and the orbital magnetic moment of Nd.