Construction of double reaction zones for long-life quasi-solid aluminum-ion batteries by realizing maximum electron transfer
Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi...
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| Published in | Nature communications Vol. 14; no. 1; pp. 5596 - 11 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
12.09.2023
Nature Publishing Group Nature Portfolio |
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| Online Access | Get full text |
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| Abstract | Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g
−1
) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs.
Achieving high energy density and long cycling life simultaneously remains a critical challenge for aluminum-ion batteries. Here, the authors develop a layered quasi-solid battery with double reaction zones to suppress shuttle effect of conversion-type materials and improve both energy density and cycling life. |
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| AbstractList | Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g
−1
) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs.
Achieving high energy density and long cycling life simultaneously remains a critical challenge for aluminum-ion batteries. Here, the authors develop a layered quasi-solid battery with double reaction zones to suppress shuttle effect of conversion-type materials and improve both energy density and cycling life. Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g −1 ) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs. Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g-1) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs.Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g-1) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs. Abstract Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g−1) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs. Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for high-capacity conversion-type positive electrodes suffering from shuttle effect in strongly acidic electrolytes. Herein, we develop a layered quasi-solid AIBs system with double reaction zones (DRZs, Zone 1 and Zone 2) to address such issues. Zone 1 is designed to accelerate reaction kinetics by improving wetting ability of quasi-solid electrolyte to active materials. A composite three-dimensional conductive framework (Zone 2) interwoven by gel network for ion conduction and carbon nanotube network as electronic conductor, can fix the active materials dissolved from Zone 1 to allow for continuing electrochemical reactions. Therefore, a maximum electron transfer is realized for the conversion-type mateials in DRZs, and an ultrahigh capacity (400 mAh g−1) and an ultralong cycling life (4000 cycles) are achieved. Such strategy provides a new perspective for constructing high-energy-density and long-life AIBs.Achieving high energy density and long cycling life simultaneously remains a critical challenge for aluminum-ion batteries. Here, the authors develop a layered quasi-solid battery with double reaction zones to suppress shuttle effect of conversion-type materials and improve both energy density and cycling life. |
| ArticleNumber | 5596 |
| Author | Wang, Zhe Song, Wei-Li Wang, Wei Jiao, Shuqiang Huang, Zheng Yu, Zhijing Zhu, Yong |
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| Snippet | Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially for... Abstract Achieving high energy density and long cycling life simultaneously remains the most critical challenge for aluminum-ion batteries (AIBs), especially... |
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| SubjectTerms | 119/118 140/146 147/135 147/143 639/301/299 Aluminum Aluminum-ion batteries Carbon nanotubes Chemical reactions Composite materials Conversion Cycles Electrochemistry Electron transfer Humanities and Social Sciences multidisciplinary Reaction kinetics Science Science (multidisciplinary) Solid electrolytes Three dimensional composites |
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| Title | Construction of double reaction zones for long-life quasi-solid aluminum-ion batteries by realizing maximum electron transfer |
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