Single atom catalysts in Van der Waals gaps

Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different in...

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Published inNature communications Vol. 13; no. 1; pp. 6863 - 9
Main Authors Jiang, Huaning, Yang, Weiwei, Xu, Mingquan, Wang, Erqing, Wei, Yi, Liu, Wei, Gu, Xiaokang, Liu, Lixuan, Chen, Qian, Zhai, Pengbo, Zou, Xiaolong, Ajayan, Pulickel M., Zhou, Wu, Gong, Yongji
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 11.11.2022
Nature Publishing Group
Nature Portfolio
Subjects
147/135
147/137
147/143
639/301/299/886
639/638/263/915
639/925/357/1018
Bonding strength
Catalysts
Catalytic activity
Chemical bonds
Chemical synthesis
Chemical vapor deposition
Durability
Electrocatalysts
Humanities and Social Sciences
Hydrogen
Hydrogen evolution reactions
Laboratories
multidisciplinary
Noble metals
Science
Science (multidisciplinary)
Single atom catalysts
Tin disulfide
Transmission electron microscopy
Two dimensional materials
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Abstract Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS 2 . The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS 2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials. A family of single-atom catalysts synthesized by intercalating metal single atoms into the van der Waals gap of two-dimensional SnS 2 is reported. The materials are applied as hydrogen evolving catalysts with good durability and overpotential.
AbstractList A family of single-atom catalysts synthesized by intercalating metal single atoms into the van der Waals gap of two-dimensional SnS2 is reported. The materials are applied as hydrogen evolving catalysts with good durability and overpotential.
Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS2. The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials.A family of single-atom catalysts synthesized by intercalating metal single atoms into the van der Waals gap of two-dimensional SnS2 is reported. The materials are applied as hydrogen evolving catalysts with good durability and overpotential.
Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS 2 . The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS 2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials. A family of single-atom catalysts synthesized by intercalating metal single atoms into the van der Waals gap of two-dimensional SnS 2 is reported. The materials are applied as hydrogen evolving catalysts with good durability and overpotential.
Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS2. The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials.Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS2. The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials.
Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to the level of their bulk metallic counterparts are grand challenges. Herein, we demonstrate a family of single-atom catalysts with different interaction types by confining metal single atoms into the van der Waals gap of two-dimensional SnS 2 . The relatively weak bonding between the noble metal single atoms and the host endows the single atoms with more intrinsic catalytic activity compared to the ones with strong chemical bonding, while the protection offered by the layered material leads to ultrahigh stability compared to the physically adsorbed single-atom catalysts on the surface. Specifically, the trace Pt-intercalated SnS 2 catalyst has superior long-term durability and comparable performance to that of commercial 10 wt% Pt/C catalyst in hydrogen evolution reaction. This work opens an avenue to explore high-performance intercalated single-atom electrocatalysts within various two-dimensional materials.
ArticleNumber 6863
Author Liu, Wei
Liu, Lixuan
Yang, Weiwei
Wang, Erqing
Zhai, Pengbo
Zhou, Wu
Ajayan, Pulickel M.
Jiang, Huaning
Wei, Yi
Gong, Yongji
Chen, Qian
Gu, Xiaokang
Xu, Mingquan
Zou, Xiaolong
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  email: yongjigong@buaa.edu.cn
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PublicationDateYYYYMMDD 2022-11-11
PublicationDate_xml – month: 11
  year: 2022
  text: 2022-11-11
  day: 11
PublicationDecade 2020
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PublicationTitle Nature communications
PublicationTitleAbbrev Nat Commun
PublicationYear 2022
Publisher Nature Publishing Group UK
Nature Publishing Group
Nature Portfolio
Publisher_xml – name: Nature Publishing Group UK
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– name: Nature Portfolio
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Snippet Single-atom catalysts provide efficiently utilized active sites to improve catalytic activities while improving the stability and enhancing the activities to...
A family of single-atom catalysts synthesized by intercalating metal single atoms into the van der Waals gap of two-dimensional SnS2 is reported. The materials...
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SubjectTerms 147/135
147/137
147/143
639/301/299/886
639/638/263/915
639/925/357/1018
Bonding strength
Catalysts
Catalytic activity
Chemical bonds
Chemical synthesis
Chemical vapor deposition
Durability
Electrocatalysts
Humanities and Social Sciences
Hydrogen
Hydrogen evolution reactions
Laboratories
multidisciplinary
Noble metals
Science
Science (multidisciplinary)
Single atom catalysts
Tin disulfide
Transmission electron microscopy
Two dimensional materials
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Title Single atom catalysts in Van der Waals gaps
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Volume 13
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