Summary of temporal changes in air dose rates and radionuclide deposition densities in the 80 km zone over five years after the Fukushima Nuclear Power Plant accident

• Published in: Journal of environmental radioactivity Vol. 210; p. 105878
• Main Authors: Saito, Kimiaki, Mikami, Satoshi, Andoh, Masaki, Matsuda, Norihiro, Kinase, Sakae, Tsuda, Shuichi, Yoshida, Tadayoshi, Sato, Tetsuro, Seki, Akiyuki, Yamamoto, Hideaki, Sanada, Yukihisa, Wainwright-Murakami, Haruko, Takemiya, Hiroshi
• Format: Journal Article
• Language: English
• Published: England Elsevier Ltd 01.12.2019
• Subjects: accidents; air; cesium; Cesium Radioisotopes; chronic exposure; decontamination; environmental monitoring; Fukushima Nuclear Accident; gamma radiation; half life; Humans; Japan; nuclear power; Nuclear Power Plants; power plants; Radiation Monitoring; radioactivity; radionuclides; Soil Pollutants, Radioactive; temporal variation; Japan
• ISSN: 0265-931X; 1879-1700; 1879-1700
• DOI: 10.1016/j.jenvrad.2018.12.020

We summarized temporal changes in air dose rates and radionuclide deposition densities over five years in the 80 km zone based on large-scale environmental monitoring data obtained continuously after the Fukushima Nuclear Power Plant (NPP) accident, including those already reported in the present and previous special issues. After the accident, multiple radionuclides deposited on the ground were detected over a wide area; radiocesium was found to be predominantly important from the viewpoint of long-term exposure. The relatively short physical half-life of 134Cs (2.06 y) has led to considerable reductions in air dose rates. The reduction in air dose rates owing to the radioactive decay of radiocesium was more than 60% over five years. Furthermore, the air dose rates in environments associated with human lives decreased at a considerably faster rate than expected for radioactive decay. The average air dose rate originating from the radiocesium deposited in the 80 km zone was lower than that predicted from radioactive decay by a factor of 2–3 at five years after the accident. Vertical penetration of radiocesium into the ground contributed greatly to the reduction in air dose rate because of an increase in the shielding of gamma rays; the estimated average reduction in air dose rate was approximately 25% with penetration compared to that without penetration. The average air dose rate measured in undisturbed fields in the 80 km zone was estimated to be reduced owing to decontamination by approximately 20% compared to that without decontamination. The average deposition density of radiocesium in undisturbed fields has decreased owing to radioactive decay, indicating that the migration of radiocesium in the horizontal direction has generally been slow. Nevertheless, in human living environments, horizontal radiocesium movement is considered to contribute significantly to the reduction in air dose rate. The contribution of horizontal radiocesium movement to the decrease in air dose rate was estimated to vary by up to 30% on average. Massive amounts of environmental data were used in extended analyses, such as the development of a predictive model or integrated air dose rate maps according to different measurement results, which facilitated clearer characterization of the contamination conditions. Ecological half-lives were evaluated in several studies by using a bi-exponential model. Short-term ecological half-lives were shorter than one year in most cases, while long-term ecological half-lives were different across the studies. Even though the general tendency of decrease in air dose rates and deposition densities in the 80 km zone were elucidated as summarized above, their trend was found to vary significantly according to location. Therefore, site-specific analysis is an important task in the future. Temporal changes in average air dose rates due to deposited radiocesium observed by large-scale measurements using different methods in the 80-km zone. [Display omitted] •Large-scale environmental monitoring elucidated temporal changes in contamination conditions in Fukushima.•Air dose rates in living environments decreased to levels lower than expected from physical decay by a factor of 2–3.•Causes of air dose rate reduction were physical decay, vertical and horizontal radiocesium movement, and decontamination.•Radiocesium movement was modified significantly by type of land use and human activity.