A Chiral, Self-Catenating and Porous Metal-Organic Framework and its Post-Synthetic Metal Uptake
Free vacancies: A robust and porous metal–organic framework material with unique 4‐connected self‐catenating structure of {85⋅10} topology was synthesized. The structure features empty bipyridine metal‐chelating sites that can be doped with copper cations in a single‐crystal‐to‐single‐crystal post‐s...
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| Published in | Angewandte Chemie International Edition Vol. 51; no. 21; pp. 5192 - 5195 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
21.05.2012
WILEY‐VCH Verlag Wiley Subscription Services, Inc |
| Edition | International ed. in English |
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| Abstract | Free vacancies: A robust and porous metal–organic framework material with unique 4‐connected self‐catenating structure of {85⋅10} topology was synthesized. The structure features empty bipyridine metal‐chelating sites that can be doped with copper cations in a single‐crystal‐to‐single‐crystal post‐synthetic modification (see picture; scale bar 20 μm). |
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| AbstractList | Free vacancies: A robust and porous metal-organic framework material with unique 4-connected self-catenating structure of {8(5) 10} topology was synthesized. The structure features empty bipyridine metal-chelating sites that can be doped with copper cations in a single-crystal-to-single-crystal post-synthetic modification (see picture; scale bar 20μm). Free vacancies: A robust and porous metal-organic framework material with unique 4-connected self-catenating structure of {8 super(5)10} topology was synthesized. The structure features empty bipyridine metal-chelating sites that can be doped with copper cations in a single-crystal-to-single-crystal post-synthetic modification (see picture; scale bar 20 mu m). Free vacancies: A robust and porous metal–organic framework material with unique 4‐connected self‐catenating structure of {85⋅10} topology was synthesized. The structure features empty bipyridine metal‐chelating sites that can be doped with copper cations in a single‐crystal‐to‐single‐crystal post‐synthetic modification (see picture; scale bar 20 μm). |
| Author | Jacobs, Tia Hardie, Michaele J. Cooper, Andrew I. Clowes, Rob |
| Author_xml | – sequence: 1 givenname: Tia surname: Jacobs fullname: Jacobs, Tia organization: School of Chemistry, University of Leeds, Woodhouse Lane, Leeds, LS2 9JT (UK) – sequence: 2 givenname: Rob surname: Clowes fullname: Clowes, Rob organization: Department of Chemistry, University of Liverpool, Liverpool, L69 7ZD (UK) – sequence: 3 givenname: Andrew I. surname: Cooper fullname: Cooper, Andrew I. organization: Department of Chemistry, University of Liverpool, Liverpool, L69 7ZD (UK) – sequence: 4 givenname: Michaele J. surname: Hardie fullname: Hardie, Michaele J. email: m.j.hardie@leeds.ac.uk organization: School of Chemistry, University of Leeds, Woodhouse Lane, Leeds, LS2 9JT (UK) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22488777$$D View this record in MEDLINE/PubMed |
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| Notes | istex:B608212CEBAB3D25BC30E1D0221427B0516378BB The Leverhulme Trust (UK) The authors thank the Diamond Light Source and S. Barnett for access to and assistance with diffraction facilities; M. A. Halcrow and J. Loughrey for assistance with ESR and A. Kulak with optical microscopy; A. Kazlauciunas for SEM-EDX measurements; I. Blakeley for microanalysis; and F. Meldrum and B. Murray for access to equipment. This work was funded by The Leverhulme Trust (UK). ark:/67375/WNG-ZF0W9C6W-S ArticleID:ANIE201200758 The authors thank the Diamond Light Source and S. Barnett for access to and assistance with diffraction facilities; M. A. Halcrow and J. Loughrey for assistance with ESR and A. Kulak with optical microscopy; A. Kazlauciunas for SEM‐EDX measurements; I. Blakeley for microanalysis; and F. Meldrum and B. Murray for access to equipment. This work was funded by The Leverhulme Trust (UK). ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 |
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| Snippet | Free vacancies: A robust and porous metal–organic framework material with unique 4‐connected self‐catenating structure of {85⋅10} topology was synthesized. The... Free vacancies: A robust and porous metal-organic framework material with unique 4-connected self-catenating structure of {8(5) 10} topology was synthesized.... Free vacancies: A robust and porous metal-organic framework material with unique 4-connected self-catenating structure of {8 super(5)10} topology was... |
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| SubjectTerms | Cations Copper metal doping Metal-organic frameworks Metals network topologies nitrogen sorption Pictures post-synthetic modification Single crystals Topology Uptakes Vacancies |
| Title | A Chiral, Self-Catenating and Porous Metal-Organic Framework and its Post-Synthetic Metal Uptake |
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