A Decade of Global Volcanic SO2 Emissions Measured from Space

• Published in: Scientific reports Vol. 7; no. 1; p. 44095
• Main Authors: Carn, S. A., Fioletov, V. E., McLinden, C. A., Li, C., Krotkov, N. A.
• Format: Journal Article
• Language: English
• Published: Goddard Space Flight Center Nature Publishing Group 09.03.2017; Nature Publishing Group UK
• Subjects: 704/106/35/824; 704/172/169/895; 704/172/4081; 704/2151/598; 704/4111; Aerosols; Atmospheric chemistry; Carbon dioxide; Climate; Climate models; Degassing; Emission inventories; Emission measurements; Emissions; Geosciences (General); Heavy metals; Humanities and Social Sciences; Islands; Mercury; Monitoring instruments; multidisciplinary; Ozone; Science; Sulfates; Sulfur; Sulfur dioxide; Trace metals; Trends; Volcanic gases; Volcanoes
• ISSN: 2045-2322; 2045-2322
• DOI: 10.1038/srep44095

The global flux of sulfur dioxide (SO2) emitted by passive volcanic degassing is a key parameter that constrains the fluxes of other volcanic gases (including carbon dioxide, CO2) and toxic trace metals (e.g., mercury). It is also a required input for atmospheric chemistry and climate models, since it impacts the tropospheric burden of sulfate aerosol, a major climate-forcing species. Despite its significance, an inventory of passive volcanic degassing is very difficult to produce, due largely to the patchy spatial and temporal coverage of ground-based SO2 measurements. We report here the first volcanic SO2 emissions inventory derived from global, coincident satellite measurements, made by the Ozone Monitoring Instrument (OMI) on NASA's Aura satellite in 2005-2015. The OMI measurements permit estimation of SO2 emissions from over 90 volcanoes, including new constraints on fluxes from Indonesia, Papua New Guinea, the Aleutian Islands, the Kuril Islands and Kamchatka. On average over the past decade, the volcanic SO2 sources consistently detected from space have discharged a total of approximately 63 kt/day SO2 during passive degassing, or approximately 23 +/- 2 Tg/yr. We find that approximately 30% of the sources show significant decadal trends in SO2 emissions, with positive trends observed at multiple volcanoes in some regions including Vanuatu, southern Japan, Peru and Chile.