Dandelion-like nickel/cobalt metal-organic framework based electrode materials for high performance supercapacitors
[Display omitted] Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hyd...
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| Published in | Journal of colloid and interface science Vol. 531; pp. 83 - 90 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
01.12.2018
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g−1 at 1 A g−1 in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g−1) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg−1 at the power density of 800 W kg−1. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs. |
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| AbstractList | Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni
and Co
, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g
at 1 A g
in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g
) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg
at the power density of 800 W kg
. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs. [Display omitted] Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g−1 at 1 A g−1 in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g−1) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg−1 at the power density of 800 W kg−1. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs. Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g-1 at 1 A g-1 in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g-1) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg-1 at the power density of 800 W kg-1. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs.Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g-1 at 1 A g-1 in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g-1) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg-1 at the power density of 800 W kg-1. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs. Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here, through modifying the molar ratio of the Ni2+ and Co2+, we have successfully fabricated Ni-MOF and Ni/Co-MOF by a facile hydrothermal method. The Ni/Co-MOF with a dandelion-like hollow structure shows an excellent specific capacitance of 758 F g−1 at 1 A g−1 in the three-electrode system. Comparing with Ni-MOF, the obtained Ni/Co-MOF has a better rate capacitance (89% retention at 10 A g−1) and cycling life (75% retention after 5000 circulations). Besides, the assembled asymmetric supercapacitor based on Ni/Co-MOF and active carbon exhibits a high specific energy density of 20.9 W h kg−1 at the power density of 800 W kg−1. All these results demonstrate that the mixed-metal strategy is an effective way to optimize the morphology and improve the electrochemical property of the MOFs. |
| Author | Gao, Shuwen Wei, Fuxiang Meng, Qingkun Ren, Yaojian Qi, Jiqiu He, Yezeng Sui, Yanwei |
| Author_xml | – sequence: 1 givenname: Shuwen surname: Gao fullname: Gao, Shuwen – sequence: 2 givenname: Yanwei surname: Sui fullname: Sui, Yanwei – sequence: 3 givenname: Fuxiang surname: Wei fullname: Wei, Fuxiang – sequence: 4 givenname: Jiqiu surname: Qi fullname: Qi, Jiqiu – sequence: 5 givenname: Qingkun surname: Meng fullname: Meng, Qingkun – sequence: 6 givenname: Yaojian surname: Ren fullname: Ren, Yaojian – sequence: 7 givenname: Yezeng surname: He fullname: He, Yezeng email: hyz0217@hotmail.com |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30025331$$D View this record in MEDLINE/PubMed |
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Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in... Metal-organic frameworks (MOFs), serving as a promising electrode material in the supercapacitors, have attracted tremendous interests in recent years. Here,... |
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| SubjectTerms | capacitance carbon cobalt coordination polymers electrochemistry electrodes hot water treatment Ni-MOF Ni/Co-MOF nickel specific energy Supercapacitors |
| Title | Dandelion-like nickel/cobalt metal-organic framework based electrode materials for high performance supercapacitors |
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