A magnon scattering platform

Significance This work describes a general scattering platform that uses magnons to explore the underlying properties of target materials. In this work we show how both phase and amplitude of magnons can be imaged using a nitrogen vacancy center magnetometer and how the scattered pattern of waves ca...

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Published inProceedings of the National Academy of Sciences - PNAS Vol. 118; no. 25; p. 1
Main Authors Zhou, Tony X., Carmiggelt, Joris J., Gächter, Lisa M., Esterlis, Ilya, Sels, Dries, Stöhr, Rainer J., Du, Chunhui, Fernandez, Daniel, Rodriguez-Nieva, Joaquin F., Büttner, Felix, Demler, Eugene, Yacoby, Amir
Format Journal Article
LanguageEnglish
Published Washington National Academy of Sciences 22.06.2021
Proceedings of the National Academy of Sciences
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Summary:Significance This work describes a general scattering platform that uses magnons to explore the underlying properties of target materials. In this work we show how both phase and amplitude of magnons can be imaged using a nitrogen vacancy center magnetometer and how the scattered pattern of waves can be used to infer geometric and magnetic properties of a target material. To demonstrate this new experimental methodology we use a permalloy disk as our target and show that even with such a simple target unexpected behavior is observed. In addition, we provide a theoretical framework to reconstruct the properties of the target. Scattering experiments have revolutionized our understanding of nature. Examples include the discovery of the nucleus [R. G. Newton, Scattering Theory of Waves and Particles (1982)], crystallography [U. Pietsch, V. Holý, T. Baumback, High-Resolution X-Ray Scattering (2004)], and the discovery of the double-helix structure of DNA [J. D. Watson, F. H. C. Crick, Nature 171, 737–738]. Scattering techniques differ by the type of particles used, the interaction these particles have with target materials, and the range of wavelengths used. Here, we demonstrate a two-dimensional table-top scattering platform for exploring magnetic properties of materials on mesoscopic length scales. Long-lived, coherent magnonic excitations are generated in a thin film of yttrium iron garnet and scattered off a magnetic target deposited on its surface. The scattered waves are then recorded using a scanning nitrogen vacancy center magnetometer that allows subwavelength imaging and operation under conditions ranging from cryogenic to ambient environment. While most scattering platforms measure only the intensity of the scattered waves, our imaging method allows for spatial determination of both amplitude and phase of the scattered waves, thereby allowing for a systematic reconstruction of the target scattering potential. Our experimental results are consistent with theoretical predictions for such a geometry and reveal several unusual features of the magnetic response of the target, including suppression near the target edges and a gradient in the direction perpendicular to the direction of surface wave propagation. Our results establish magnon scattering experiments as a platform for studying correlated many-body systems.
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SC0001819; SC0019300; W911NF-17-1-0023; W911NF-1-81-0206; FA95501610323; D18AC00014; 820394; GBMF4531; FA9500-20-1-0319; EFMA-1542807; ECCS-1541959
European Union (EU)
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
US Army Research Office (ARO)
USDOE
Gordon and Betty Moore Foundation
Netherlands Organisation for Scientific Research
National Science Foundation (NSF)
US Air Force Office of Scientific Research (AFOSR)
Author contributions: T.X.Z. and A.Y. conceived the idea and the project; T.X.Z. led the project; T.X.Z., J.J.C., L.M.G., and A.Y. designed the phase measurement schemes and performed the phase imaging research; T.X.Z. fabricated the scanning probes; T.X.Z., L.M.G., R.J.S., and D.F. built the scanning probe setup; T.X.Z., I.E., D.S., E.D., and A.Y. designed scattering theory; I.E., D.S., E.D., and A.Y. developed the scattering theory; C.D. contributed discussion and methods used from previous generation of experiments; J.F.R.-N. contributed discussion and knowledge from previous understanding of theory; F.B. contributed discussion about magnetic imaging technique; T.X.Z., J.J.C., L.M.G., I.E., D.S., E.D., and A.Y. wrote the manuscript with input from R.J.S., C.D., D.F., J.F.R.-N., and F.B.; and A.Y. supervised the project.
Reviewers: M.E.F., The University of Iowa; and J.S., Texas A&M University.
1T.X.Z., J.J.C., and L.M.G. contributed equally to this work.
Contributed by Amir Yacoby, April 19, 2021 (sent for review September 16, 2020; reviewed by Michael E. Flatté and Jairo Sinova)
ISSN:0027-8424
1091-6490
DOI:10.1073/pnas.2019473118