A Study: Removal of Cu(II), Cd(II), and Pb(II) Ions from Real Industrial Water and Contaminated Water Using Activated Sludge Biomass
This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion‐exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of...
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Published in | Clean : soil, air, water Vol. 40; no. 11; pp. 1273 - 1283 |
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WILEY-VCH Verlag
01.11.2012
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Abstract | This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion‐exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of 6.0 based on its monolayer capacities. Maximum monolayer capacities of AS biomass (qmax) were calculated as 0.478, 0.358, and 0.280 mmol g−1 for Cu2+, Cd2+, and Pb2+, respectively, and the adsorption equilibrium time was found as 60 min for each metal. The adsorbed amount of metal rose with increasing of initial metal ion concentration. The equilibrium adsorption capacity of AS for initial 0.25 mmol L−1 metal concentration was determined as 0.200, 0.167, and 0.155 mmol g−1 for Cu2+, Cd2+, and Pb2+ ions, respectively. These relevant values were determined as 0.420, 0.305, and 0.282 mmol g−1 for Cu2+, Cd2+, and Pb2+ ions, respectively, when initial metal concentration was 0.50 mmol L−1. In the multi‐metal sorption system, the adsorption capacity of AS biomass was observed in the order of Cu2+ > Cd2+ > Pb2+. In the presence of 100 mmol L−1 H+ ion, the order of ion‐exchange affinity with H+ was found as Cu2+ > Cd2+ > Pb2+. The adsorption kinetics were also found to be well described by the pseudo‐second‐order and intraparticle diffusion models. Two different rate constants were obtained as ki1 and ki2 and ki1 (first stage) was found to be higher than ki2 (second stage).
The results of the FTIR analysis indicated that AS biomass has –OH, –NH2, –COOH, and –PO4 groups which can react with Cu2+, Cd2+, and Pb2+ ions. The dried AS could be a promising and cheap alternative for the treatment of pure and industrial wastewater. |
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AbstractList | This study aims to remove of Cu super(2+), Cd super(2+), and Pb super(2+) ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion-exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of 6.0 based on its monolayer capacities. Maximum monolayer capacities of AS biomass (q sub(max)) were calculated as 0.478, 0.358, and 0.280mmolg super(-1) for Cu super(2+), Cd super(2+), and Pb super(2+), respectively, and the adsorption equilibrium time was found as 60min for each metal. The adsorbed amount of metal rose with increasing of initial metal ion concentration. The equilibrium adsorption capacity of AS for initial 0.25mmolL super(-1) metal concentration was determined as 0.200, 0.167, and 0.155mmolg super(-1) for Cu super(2+), Cd super(2+), and Pb super(2+) ions, respectively. These relevant values were determined as 0.420, 0.305, and 0.282mmolg super(-1) for Cu super(2+), Cd super(2+), and Pb super(2+) ions, respectively, when initial metal concentration was 0.50mmolL super(-1). In the multi-metal sorption system, the adsorption capacity of AS biomass was observed in the order of Cu super(2+)>Cd super(2+)>Pb super(2+). In the presence of 100mmolL super(-1) H super(+) ion, the order of ion-exchange affinity with H super(+) was found as Cu super(2+)>Cd super(2+)>Pb super(2+). The adsorption kinetics were also found to be well described by the pseudo-second-order and intraparticle diffusion models. Two different rate constants were obtained as k sub(i1) and k sub(i2) and k sub(i1) (first stage) was found to be higher than k sub(i2) (second stage). The results of the FTIR analysis indicated that AS biomass has -OH, -NH sub(2), -COOH, and -PO sub(4) groups which can react with Cu super(2+), Cd super(2+), and Pb super(2+) ions. The dried AS could be a promising and cheap alternative for the treatment of pure and industrial wastewater. Abstract This study aims to remove of Cu 2+ , Cd 2+ , and Pb 2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion‐exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of 6.0 based on its monolayer capacities. Maximum monolayer capacities of AS biomass ( q max ) were calculated as 0.478, 0.358, and 0.280 mmol g −1 for Cu 2+ , Cd 2+ , and Pb 2+ , respectively, and the adsorption equilibrium time was found as 60 min for each metal. The adsorbed amount of metal rose with increasing of initial metal ion concentration. The equilibrium adsorption capacity of AS for initial 0.25 mmol L −1 metal concentration was determined as 0.200, 0.167, and 0.155 mmol g −1 for Cu 2+ , Cd 2+ , and Pb 2+ ions, respectively. These relevant values were determined as 0.420, 0.305, and 0.282 mmol g −1 for Cu 2+ , Cd 2+ , and Pb 2+ ions, respectively, when initial metal concentration was 0.50 mmol L −1 . In the multi‐metal sorption system, the adsorption capacity of AS biomass was observed in the order of Cu 2+ > Cd 2+ > Pb 2+ . In the presence of 100 mmol L −1 H + ion, the order of ion‐exchange affinity with H + was found as Cu 2+ > Cd 2+ > Pb 2+ . The adsorption kinetics were also found to be well described by the pseudo‐second‐order and intraparticle diffusion models. Two different rate constants were obtained as k i1 and k i2 and k i1 (first stage) was found to be higher than k i2 (second stage). This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion‐exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of 6.0 based on its monolayer capacities. Maximum monolayer capacities of AS biomass (qmax) were calculated as 0.478, 0.358, and 0.280 mmol g−1 for Cu2+, Cd2+, and Pb2+, respectively, and the adsorption equilibrium time was found as 60 min for each metal. The adsorbed amount of metal rose with increasing of initial metal ion concentration. The equilibrium adsorption capacity of AS for initial 0.25 mmol L−1 metal concentration was determined as 0.200, 0.167, and 0.155 mmol g−1 for Cu2+, Cd2+, and Pb2+ ions, respectively. These relevant values were determined as 0.420, 0.305, and 0.282 mmol g−1 for Cu2+, Cd2+, and Pb2+ ions, respectively, when initial metal concentration was 0.50 mmol L−1. In the multi‐metal sorption system, the adsorption capacity of AS biomass was observed in the order of Cu2+ > Cd2+ > Pb2+. In the presence of 100 mmol L−1 H+ ion, the order of ion‐exchange affinity with H+ was found as Cu2+ > Cd2+ > Pb2+. The adsorption kinetics were also found to be well described by the pseudo‐second‐order and intraparticle diffusion models. Two different rate constants were obtained as ki1 and ki2 and ki1 (first stage) was found to be higher than ki2 (second stage). The results of the FTIR analysis indicated that AS biomass has –OH, –NH2, –COOH, and –PO4 groups which can react with Cu2+, Cd2+, and Pb2+ ions. The dried AS could be a promising and cheap alternative for the treatment of pure and industrial wastewater. This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion-exchange affinities of these metals using waste activated sludge (AS) biomass. The adsorptions of the metals on biomass were optimal at an acidic pH value of 6.0 based on its monolayer capacities. Maximum monolayer capacities of AS biomass (qmax) were calculated as 0.478, 0.358, and 0.280mmolg-1 for Cu2+, Cd2+, and Pb2+, respectively, and the adsorption equilibrium time was found as 60min for each metal. The adsorbed amount of metal rose with increasing of initial metal ion concentration. The equilibrium adsorption capacity of AS for initial 0.25mmolL-1 metal concentration was determined as 0.200, 0.167, and 0.155mmolg-1 for Cu2+, Cd2+, and Pb2+ ions, respectively. These relevant values were determined as 0.420, 0.305, and 0.282mmolg-1 for Cu2+, Cd2+, and Pb2+ ions, respectively, when initial metal concentration was 0.50mmolL-1. In the multi-metal sorption system, the adsorption capacity of AS biomass was observed in the order of Cu2+>Cd2+>Pb2+. In the presence of 100mmolL-1 H+ ion, the order of ion-exchange affinity with H+ was found as Cu2+>Cd2+>Pb2+. The adsorption kinetics were also found to be well described by the pseudo-second-order and intraparticle diffusion models. Two different rate constants were obtained as ki1 and ki2 and ki1 (first stage) was found to be higher than ki2 (second stage). |
Author | Gulnaz, Osman Samil, Ali Kusvuran, Erdal Yildirim, Deniz |
Author_xml | – sequence: 1 givenname: Erdal surname: Kusvuran fullname: Kusvuran, Erdal email: erdalkusvuran@yahoo.com, ekusvuran@cu.edu.tr organization: Arts and Sciences Faculty, Chemistry Department, Cukurova University, Balcali, Adana, Turkey – sequence: 2 givenname: Deniz surname: Yildirim fullname: Yildirim, Deniz organization: Arts and Sciences Faculty, Chemistry Department, Cukurova University, Balcali, Adana, Turkey – sequence: 3 givenname: Ali surname: Samil fullname: Samil, Ali organization: Arts and Sciences Faculty, Chemistry Department, Sutcu Imam University, Kahramanmaras, Turkey – sequence: 4 givenname: Osman surname: Gulnaz fullname: Gulnaz, Osman organization: Arts and Sciences Faculty, Biology Department, Cukurova University, Balcali, Adana, Turkey |
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Snippet | This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion‐exchange... Abstract This study aims to remove of Cu 2+ , Cd 2+ , and Pb 2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and... This study aims to remove of Cu2+, Cd2+, and Pb2+ ions from solution and to investigate the adsorption isotherms, adsorption kinetics, and ion-exchange... This study aims to remove of Cu super(2+), Cd super(2+), and Pb super(2+) ions from solution and to investigate the adsorption isotherms, adsorption kinetics,... |
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SubjectTerms | Adsorption Biomass Earth sciences Earth, ocean, space Exact sciences and technology FTIR Heavy metal Hydrology Hydrology. Hydrogeology Kinetic models Multi metal sorption system Water treatment |
Title | A Study: Removal of Cu(II), Cd(II), and Pb(II) Ions from Real Industrial Water and Contaminated Water Using Activated Sludge Biomass |
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