Aerosol particle formation in the upper residual layer

• Published in: Atmospheric chemistry and physics Vol. 21; no. 10; pp. 7901 - 7915
• Main Authors: Lampilahti, Janne, Leino, Katri, Manninen, Antti, Poutanen, Pyry, Franck, Anna, Peltola, Maija, Hietala, Paula, Beck, Lisa, Dada, Lubna, Quéléver, Lauriane, Öhrnberg, Ronja, Zhou, Ying, Ekblom, Madeleine, Vakkari, Ville, Zilitinkevich, Sergej, Kerminen, Veli-Matti, Petäjä, Tuukka, Kulmala, Markku
• Format: Journal Article
• Language: English
• Published: Katlenburg-Lindau Copernicus GmbH 25.05.2021; Copernicus Publications
• Subjects: Aerosol particles; Aerosols; Airborne sensing; Aircraft; Altitude; Atmospheric boundary layer; Boreal forests; Boundary layers; Cloud condensation nuclei; Clouds; Condensation nuclei; Earth atmosphere; Hypotheses; Lower troposphere; Mixed layer; Particle formation; Taiga; Troposphere; United States > US; Finland
• ISSN: 1680-7324; 1680-7316; 1680-7324
• DOI: 10.5194/acp-21-7901-2021

According to current estimates, atmospheric new particle formation (NPF) produces a large fraction of aerosol particles and cloud condensation nuclei in the Earth's atmosphere, which have implications for health and climate. Despite recent advances, atmospheric NPF is still insufficiently understood in the lower troposphere, especially above the mixed layer (ML). This paper presents new results from co-located airborne and ground-based measurements in a boreal forest environment, showing that many NPF events (∼42 %) appear to start in the topmost part of the residual layer (RL). The freshly formed particles may be entrained into the growing mixed layer (ML) where they continue to grow in size, similar to the aerosol particles formed within the ML. The results suggest that in the boreal forest environment, NPF in the upper RL has an important contribution to the aerosol load in the boundary layer (BL).