A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal–Organic Frameworks

Blue‐color stimulated emission with low threshold power is observed from In‐ and Zn‐MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal‐ion centers in the solid state. The density‐of‐states and transition dipole moments are calculated and the stimulate...

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Published inAdvanced materials (Weinheim) Vol. 29; no. 17
Main Authors Medishetty, Raghavender, Nalla, Venkatram, Nemec, Lydia, Henke, Sebastian, Mayer, David, Sun, Handong, Reuter, Karsten, Fischer, Roland A.
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.05.2017
Subjects
blue emission
Color
Density of states
Dipole moments
Fluorescence
hybrid materials
Lasing
Materials science
Metal-organic frameworks
nonlinear optics
Optical activity
Solid state
Stimulated emission
two‐photon excited fluorescence
blue emission
nonlinear optics
hybrid materials
two-photon excited fluorescence
stimulated emission
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Summary:Blue‐color stimulated emission with low threshold power is observed from In‐ and Zn‐MOFs, which feature a highly fluorescent chromophore densely packed and rigidly linked to the metal‐ion centers in the solid state. The density‐of‐states and transition dipole moments are calculated and the stimulated emission phenomenon is correlated with these properties.
Bibliography:ObjectType-Article-1
SourceType-Scholarly Journals-1
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content type line 23
ISSN:0935-9648
1521-4095
DOI:10.1002/adma.201605637