Recent Advances of Porous Graphene: Synthesis, Functionalization, and Electrochemical Applications

Graphene is a 2D sheet of sp2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these is...

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Published inSmall (Weinheim an der Bergstrasse, Germany) Vol. 15; no. 48; pp. e1903780 - n/a
Main Authors Zhang, Yuanyuan, Wan, Qijin, Yang, Nianjun
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.11.2019
Subjects
Bonding strength
Chemical bonds
Composite materials
electrochemical applications
Energy storage
functionalization
Graphene
Mass transfer
Nanotechnology
porous graphene
Synthesis
functionalization
synthesis
electrochemical applications
porous graphene
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Abstract Graphene is a 2D sheet of sp2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these issues, various kinds of 2D holey graphene and 3D porous graphene are either self‐assembled from graphene layers or fabricated using graphene related materials such as graphene oxide and reduced graphene oxide. Porous graphene not only possesses unique pore structures, but also introduces abundant exposed edges and accelerates mass transfer. The properties and applications of these porous graphenes and their composites/hybrids have been extensively studied in recent years. Herein, recent progress and achievements in synthesis and functionalization of various 2D holey graphene and 3D porous graphene are reviewed. Of special interest, electrochemical applications of porous graphene and its hybrids in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage, are highlighted. As the closing remarks, the challenges and opportunities for the future research of porous graphene and its composites are discussed and outlined. Synthesis of 2D and 3D porous graphene is reviewed together with their functionalization with hetero‐atoms and other functional materials. Electrochemical applications of these porous graphene are highlighted in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage and conversion. The future research directions and challenges on porous graphene are also discussed and outlined.
AbstractList Abstract Graphene is a 2D sheet of sp 2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these issues, various kinds of 2D holey graphene and 3D porous graphene are either self‐assembled from graphene layers or fabricated using graphene related materials such as graphene oxide and reduced graphene oxide. Porous graphene not only possesses unique pore structures, but also introduces abundant exposed edges and accelerates mass transfer. The properties and applications of these porous graphenes and their composites/hybrids have been extensively studied in recent years. Herein, recent progress and achievements in synthesis and functionalization of various 2D holey graphene and 3D porous graphene are reviewed. Of special interest, electrochemical applications of porous graphene and its hybrids in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage, are highlighted. As the closing remarks, the challenges and opportunities for the future research of porous graphene and its composites are discussed and outlined.
Graphene is a 2D sheet of sp2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these issues, various kinds of 2D holey graphene and 3D porous graphene are either self‐assembled from graphene layers or fabricated using graphene related materials such as graphene oxide and reduced graphene oxide. Porous graphene not only possesses unique pore structures, but also introduces abundant exposed edges and accelerates mass transfer. The properties and applications of these porous graphenes and their composites/hybrids have been extensively studied in recent years. Herein, recent progress and achievements in synthesis and functionalization of various 2D holey graphene and 3D porous graphene are reviewed. Of special interest, electrochemical applications of porous graphene and its hybrids in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage, are highlighted. As the closing remarks, the challenges and opportunities for the future research of porous graphene and its composites are discussed and outlined.
Graphene is a 2D sheet of sp2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these issues, various kinds of 2D holey graphene and 3D porous graphene are either self‐assembled from graphene layers or fabricated using graphene related materials such as graphene oxide and reduced graphene oxide. Porous graphene not only possesses unique pore structures, but also introduces abundant exposed edges and accelerates mass transfer. The properties and applications of these porous graphenes and their composites/hybrids have been extensively studied in recent years. Herein, recent progress and achievements in synthesis and functionalization of various 2D holey graphene and 3D porous graphene are reviewed. Of special interest, electrochemical applications of porous graphene and its hybrids in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage, are highlighted. As the closing remarks, the challenges and opportunities for the future research of porous graphene and its composites are discussed and outlined. Synthesis of 2D and 3D porous graphene is reviewed together with their functionalization with hetero‐atoms and other functional materials. Electrochemical applications of these porous graphene are highlighted in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage and conversion. The future research directions and challenges on porous graphene are also discussed and outlined.
Graphene is a 2D sheet of sp bonded carbon atoms and tends to aggregate together, due to the strong π-π stacking and van der Waals attraction between different layers. Its unique properties such as a high specific surface area and a fast mass transport rate are severely blocked. To address these issues, various kinds of 2D holey graphene and 3D porous graphene are either self-assembled from graphene layers or fabricated using graphene related materials such as graphene oxide and reduced graphene oxide. Porous graphene not only possesses unique pore structures, but also introduces abundant exposed edges and accelerates mass transfer. The properties and applications of these porous graphenes and their composites/hybrids have been extensively studied in recent years. Herein, recent progress and achievements in synthesis and functionalization of various 2D holey graphene and 3D porous graphene are reviewed. Of special interest, electrochemical applications of porous graphene and its hybrids in the fields of electrochemical sensing, electrocatalysis, and electrochemical energy storage, are highlighted. As the closing remarks, the challenges and opportunities for the future research of porous graphene and its composites are discussed and outlined.
Author Zhang, Yuanyuan
Yang, Nianjun
Wan, Qijin
Author_xml – sequence: 1
  givenname: Yuanyuan
  surname: Zhang
  fullname: Zhang, Yuanyuan
  email: yyzhang@wit.edu.cn
  organization: Wuhan Institute of Technology
– sequence: 2
  givenname: Qijin
  surname: Wan
  fullname: Wan, Qijin
  organization: Wuhan Institute of Technology
– sequence: 3
  givenname: Nianjun
  orcidid: 0000-0002-5558-2314
  surname: Yang
  fullname: Yang, Nianjun
  email: nianjun.yang@uni-siegen.de
  organization: University of Siegen
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31663294$$D View this record in MEDLINE/PubMed
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Keywords functionalization
synthesis
electrochemical applications
porous graphene
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Snippet Graphene is a 2D sheet of sp2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction between...
Graphene is a 2D sheet of sp bonded carbon atoms and tends to aggregate together, due to the strong π-π stacking and van der Waals attraction between different...
Abstract Graphene is a 2D sheet of sp 2 bonded carbon atoms and tends to aggregate together, due to the strong π–π stacking and van der Waals attraction...
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StartPage e1903780
SubjectTerms Bonding strength
Chemical bonds
Composite materials
electrochemical applications
Energy storage
functionalization
Graphene
Mass transfer
Nanotechnology
porous graphene
Synthesis
Title Recent Advances of Porous Graphene: Synthesis, Functionalization, and Electrochemical Applications
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fsmll.201903780
https://www.ncbi.nlm.nih.gov/pubmed/31663294
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Volume 15
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