Dynamics and mass transfer of rising bubbles in a homogenous swarm at large gas volume fraction

• Published in: Journal of fluid mechanics Vol. 763; pp. 254 - 285
• Main Authors: Colombet, Damien, Legendre, Dominique, Risso, Frédéric, Cockx, Arnaud, Guiraud, Pascal
• Format: Journal Article
• Language: English
• Published: Cambridge, UK Cambridge University Press 01.01.2015; Cambridge University Press (CUP)
• Subjects: Bubbles; Diffusion coefficient; Fluid mechanics; Gases; Life Sciences; Mass transfer; Velocity; Water; drops and bubbles; bubble dynamics; IN-LINE; Agitation; HEAT-TRANSFER; VOFRACTION; LIQUID; PACKED-BEDS; STIRRED-TANK; Mass transfer; CHEMICAL-REACTIONS; REYNOLDS-NUMBER; Bubbly flow; 2 SPHERICAL BUBBLES; VELOCITY FLUCTUATIONS
• ISSN: 0022-1120; 1469-7645
• DOI: 10.1017/jfm.2014.672

The present work focuses on the collective effect on both bubble dynamics and mass transfer in a dense homogeneous bubble swarm for gas volume fractions ${\it\alpha}$ up to 30 %. The experimental investigation is carried out with air bubbles rising in a square column filled with water. Bubble size and shape are determined by means of a high-speed camera equipped with a telecentric lens. Gas volume fraction and bubble velocity are measured by using a dual-tip optical probe. The combination of these two techniques allows us to determine the interfacial area between the gas and the liquid. The transfer of oxygen from the bubbles to the water is measured from the time evolution of the concentration of oxygen dissolved in water, which is obtained by means of the gassing-out method. Concerning the bubble dynamics, the average vertical velocity is observed to decrease with ${\it\alpha}$ in agreement with previous experimental and numerical investigations, while the bubble agitation turns out to be weakly dependent on  ${\it\alpha}$ . Concerning mass transfer, the Sherwood number is found to be very close to that of a single bubble rising at the same Reynolds number, provided the latter is based on the average vertical bubble velocity, which accounts for the effect of the gas volume fraction on the bubble rise velocity. This conclusion is valid for situations where the diffusion coefficient of the gas in the liquid is very low (high Péclet number) and the dissolved gas is well mixed at the scale of the bubble. It is understood by considering that the transfer occurs at the front part of the bubbles through a diffusion layer which is very thin compared with all flow length scales and where the flow remains similar to that of a single rising bubble.