Functional manganese ferrite/graphene oxide nanocomposites: effects of graphene oxide on the adsorption mechanisms of organic MB dye and inorganic As(v) ions from aqueous solution

In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomp...

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Published inRSC advances Vol. 8; no. 22; pp. 12376 - 12389
Main Authors Lan Huong, Pham Thi, Tu, Nguyen, Lan, Hoang, Thang, Le Hong, Van Quy, Nguyen, Tuan, Pham Anh, Dinh, Ngo Xuan, Phan, Vu Ngoc, Le, Anh-Tuan
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 01.01.2018
The Royal Society of Chemistry
Subjects
Adsorbates
Adsorption
Aqueous solutions
Arsenic
Binding sites
Chemical precipitation
Chemistry
Computer simulation
Conjugation
Dyes
Ferrites
Functional groups
Graphene
Heavy metals
Ionic interactions
Isotherms
Magnetic properties
Manganese ions
Methylene blue
Nanocomposites
Pollutants
Online AccessGet full text

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Abstract In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomposites were studied. Methylene blue (MB) and arsenic( v ) were used in this study as model water pollutants. With an increase in the GO content in the range of 10 wt% to 50 wt%, the removal efficiency for both MB dye and arsenic( v ) ions was improved. Our adsorption data revealed that the adsorption behavior of MB dye showed good agreement with the Langmuir isotherm model and pseudo-second-order equation, whereas the Freundlich isotherm model was more suitable for simulating the adsorption process of arsenic( v ) ions on the MFO-GO nanocomposites. In addition, an important role of the GO content in the adsorption mechanisms of both MB dye and arsenic( v ) ions was found, in which GO nanosheets play a key role in the mechanisms of electrostatic/ionic interactions, oxygen-containing groups and π-π conjugation in the case of the adsorption of MB dye, whereas the role of the GO content is mainly related to the mechanism of electrostatic/ionic interactions in the case of the adsorption of arsenic( v ). Graphene oxide has the functions of increasing the number of active binding sites comprising oxygen-containing functional groups, reducing the agglomeration of MFO nanoparticles, increasing the number of adsorption sites, and improving the electrostatic/ionic interactions between adsorbents and adsorbates in order to enhance the adsorption performance of cationic organic dyes and/or heavy metal anions from aqueous solutions. In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension.
AbstractList In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe3+ and Mn2+ ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomposites were studied. Methylene blue (MB) and arsenic(v) were used in this study as model water pollutants. With an increase in the GO content in the range of 10 wt% to 50 wt%, the removal efficiency for both MB dye and arsenic(v) ions was improved. Our adsorption data revealed that the adsorption behavior of MB dye showed good agreement with the Langmuir isotherm model and pseudo-second-order equation, whereas the Freundlich isotherm model was more suitable for simulating the adsorption process of arsenic(v) ions on the MFO-GO nanocomposites. In addition, an important role of the GO content in the adsorption mechanisms of both MB dye and arsenic(v) ions was found, in which GO nanosheets play a key role in the mechanisms of electrostatic/ionic interactions, oxygen-containing groups and π–π conjugation in the case of the adsorption of MB dye, whereas the role of the GO content is mainly related to the mechanism of electrostatic/ionic interactions in the case of the adsorption of arsenic(v). Graphene oxide has the functions of increasing the number of active binding sites comprising oxygen-containing functional groups, reducing the agglomeration of MFO nanoparticles, increasing the number of adsorption sites, and improving the electrostatic/ionic interactions between adsorbents and adsorbates in order to enhance the adsorption performance of cationic organic dyes and/or heavy metal anions from aqueous solutions.
In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomposites were studied. Methylene blue (MB) and arsenic( v ) were used in this study as model water pollutants. With an increase in the GO content in the range of 10 wt% to 50 wt%, the removal efficiency for both MB dye and arsenic( v ) ions was improved. Our adsorption data revealed that the adsorption behavior of MB dye showed good agreement with the Langmuir isotherm model and pseudo-second-order equation, whereas the Freundlich isotherm model was more suitable for simulating the adsorption process of arsenic( v ) ions on the MFO-GO nanocomposites. In addition, an important role of the GO content in the adsorption mechanisms of both MB dye and arsenic( v ) ions was found, in which GO nanosheets play a key role in the mechanisms of electrostatic/ionic interactions, oxygen-containing groups and π–π conjugation in the case of the adsorption of MB dye, whereas the role of the GO content is mainly related to the mechanism of electrostatic/ionic interactions in the case of the adsorption of arsenic( v ). Graphene oxide has the functions of increasing the number of active binding sites comprising oxygen-containing functional groups, reducing the agglomeration of MFO nanoparticles, increasing the number of adsorption sites, and improving the electrostatic/ionic interactions between adsorbents and adsorbates in order to enhance the adsorption performance of cationic organic dyes and/or heavy metal anions from aqueous solutions.
In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared a co-precipitation reaction of Fe and Mn ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomposites were studied. Methylene blue (MB) and arsenic(v) were used in this study as model water pollutants. With an increase in the GO content in the range of 10 wt% to 50 wt%, the removal efficiency for both MB dye and arsenic(v) ions was improved. Our adsorption data revealed that the adsorption behavior of MB dye showed good agreement with the Langmuir isotherm model and pseudo-second-order equation, whereas the Freundlich isotherm model was more suitable for simulating the adsorption process of arsenic(v) ions on the MFO-GO nanocomposites. In addition, an important role of the GO content in the adsorption mechanisms of both MB dye and arsenic(v) ions was found, in which GO nanosheets play a key role in the mechanisms of electrostatic/ionic interactions, oxygen-containing groups and π-π conjugation in the case of the adsorption of MB dye, whereas the role of the GO content is mainly related to the mechanism of electrostatic/ionic interactions in the case of the adsorption of arsenic(v). Graphene oxide has the functions of increasing the number of active binding sites comprising oxygen-containing functional groups, reducing the agglomeration of MFO nanoparticles, increasing the number of adsorption sites, and improving the electrostatic/ionic interactions between adsorbents and adsorbates in order to enhance the adsorption performance of cationic organic dyes and/or heavy metal anions from aqueous solutions.
In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension. The effects of graphene oxide on the physicochemical characteristics, magnetic properties and adsorption activities of the MFO-GO nanocomposites were studied. Methylene blue (MB) and arsenic( v ) were used in this study as model water pollutants. With an increase in the GO content in the range of 10 wt% to 50 wt%, the removal efficiency for both MB dye and arsenic( v ) ions was improved. Our adsorption data revealed that the adsorption behavior of MB dye showed good agreement with the Langmuir isotherm model and pseudo-second-order equation, whereas the Freundlich isotherm model was more suitable for simulating the adsorption process of arsenic( v ) ions on the MFO-GO nanocomposites. In addition, an important role of the GO content in the adsorption mechanisms of both MB dye and arsenic( v ) ions was found, in which GO nanosheets play a key role in the mechanisms of electrostatic/ionic interactions, oxygen-containing groups and π-π conjugation in the case of the adsorption of MB dye, whereas the role of the GO content is mainly related to the mechanism of electrostatic/ionic interactions in the case of the adsorption of arsenic( v ). Graphene oxide has the functions of increasing the number of active binding sites comprising oxygen-containing functional groups, reducing the agglomeration of MFO nanoparticles, increasing the number of adsorption sites, and improving the electrostatic/ionic interactions between adsorbents and adsorbates in order to enhance the adsorption performance of cationic organic dyes and/or heavy metal anions from aqueous solutions. In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO suspension.
Author Dinh, Ngo Xuan
Lan, Hoang
Tuan, Pham Anh
Le, Anh-Tuan
Phan, Vu Ngoc
Lan Huong, Pham Thi
Tu, Nguyen
Thang, Le Hong
Van Quy, Nguyen
AuthorAffiliation Hanoi University of Science and Technology (HUST)
Advanced Institute for Science and Technology (AIST)
International Training Institute for Materials Science (ITIMS)
Vietnam Metrology Institute
School of Materials Science and Engineering
University of Transport Technology
Saigon University (SGU)
Department of Nanoscience and Nanotechnology
Hanoi University of Science and Technology
AuthorAffiliation_xml – name: University of Transport Technology
– name: Saigon University (SGU)
– name: Advanced Institute for Science and Technology (AIST)
– name: International Training Institute for Materials Science (ITIMS)
– name: School of Materials Science and Engineering
– name: Hanoi University of Science and Technology (HUST)
– name: Hanoi University of Science and Technology
– name: Vietnam Metrology Institute
– name: Department of Nanoscience and Nanotechnology
Author_xml – sequence: 1
  givenname: Pham Thi
  surname: Lan Huong
  fullname: Lan Huong, Pham Thi
– sequence: 2
  givenname: Nguyen
  surname: Tu
  fullname: Tu, Nguyen
– sequence: 3
  givenname: Hoang
  surname: Lan
  fullname: Lan, Hoang
– sequence: 4
  givenname: Le Hong
  surname: Thang
  fullname: Thang, Le Hong
– sequence: 5
  givenname: Nguyen
  surname: Van Quy
  fullname: Van Quy, Nguyen
– sequence: 6
  givenname: Pham Anh
  surname: Tuan
  fullname: Tuan, Pham Anh
– sequence: 7
  givenname: Ngo Xuan
  surname: Dinh
  fullname: Dinh, Ngo Xuan
– sequence: 8
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  surname: Phan
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– sequence: 9
  givenname: Anh-Tuan
  surname: Le
  fullname: Le, Anh-Tuan
BackLink https://www.ncbi.nlm.nih.gov/pubmed/35539375$$D View this record in MEDLINE/PubMed
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Snippet In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe 3+ and Mn 2+ ions in a GO...
In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared a co-precipitation reaction of Fe and Mn ions in a GO suspension. The...
In this study, manganese ferrite-graphene oxide (MFO-GO) nanocomposites were prepared via a co-precipitation reaction of Fe3+ and Mn2+ ions in a GO suspension....
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SubjectTerms Adsorbates
Adsorption
Aqueous solutions
Arsenic
Binding sites
Chemical precipitation
Chemistry
Computer simulation
Conjugation
Dyes
Ferrites
Functional groups
Graphene
Heavy metals
Ionic interactions
Isotherms
Magnetic properties
Manganese ions
Methylene blue
Nanocomposites
Pollutants
Title Functional manganese ferrite/graphene oxide nanocomposites: effects of graphene oxide on the adsorption mechanisms of organic MB dye and inorganic As(v) ions from aqueous solution
URI https://www.ncbi.nlm.nih.gov/pubmed/35539375
https://www.proquest.com/docview/2021476887
https://search.proquest.com/docview/2662544953
https://pubmed.ncbi.nlm.nih.gov/PMC9079275
Volume 8
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