Ceramic foam substrates for automotive catalyst applications: fluid mechanic analysis

• Published in: Experiments in fluids Vol. 47; no. 2; pp. 209 - 222
• Main Authors: Dimopoulos Eggenschwiler, Panayotis, Tsinoglou, Dimitrios N., Seyfert, Jacqueline, Bach, Christian, Vogt, Ulrich, Gorbar, Michal
• Format: Journal Article
• Language: English
• Published: Berlin/Heidelberg Springer-Verlag 01.08.2009; Springer
• Subjects: Air pollution caused by fuel industries; Applied sciences; Atmospheric pollution; Automotive engineering; Catalysis; Catalysts: preparations and properties; Ceramics; Chemistry; Energy; Energy. Thermal use of fuels; Engineering; Engineering Fluid Dynamics; Engineering Thermodynamics; Exact sciences and technology; Fluid dynamics; Fluid flow; Fluid- and Aerodynamics; Foams; Fundamental areas of phenomenology (including applications); General and physical chemistry; Heat and Mass Transfer; Homogenizing; Honeycomb; Instrumentation for fluid dynamics; Physics; Pollution; Pollution reduction; Pressure drop; Prevention and purification methods; Research Article; Stack gas and industrial effluent processing; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry; Transports and other; Variability; Mass Flow Rate; Pressure Drop; Selective Catalytic Reduction; Foam; Particle Image Velocimetry; Fluid mechanics; Motor car; Speed measurement; Motor vehicle; Experimental study; Supported catalyst; Porous medium flow; Catalytic converter; Test facility; Pressure drop; Particle image velocimetry; Physicochemical purification; Exhaust gas; Ceramic materials; Flue gas purification
• ISSN: 0723-4864; 1432-1114
• DOI: 10.1007/s00348-009-0653-2

Several properties of ceramic foams render them promising substrates for various industrial processes. For automotive applications, the foam properties that need to be further studied include the substrate impact on the exhaust gas flow, in terms of pressure drop and flow uniformity. In this paper, pressure drop measurements are performed with different honeycomb and ceramic foam substrates, and pressure drop correlations are discussed. The flow uniformity upstream and downstream of the substrates is evaluated using particle image velocimetry. The results show that ceramic foam substrates induce higher pressure drop, while increasing the uniformity of the flow. In contrast to honeycomb monoliths, the flow uniformity downstream of ceramic foams does not decrease with increasing flow velocity. The higher flow uniformity of ceramic foams is not only caused by their higher pressure drop, but also by flow homogenization that occurs inside the ceramic foam structure, as a result of the momentum exchange perpendicular to the main flow direction.