Conjugated polymer donor-molecular acceptor nanohybrids for photocatalytic hydrogen evolution

A library of 237 organic binary/ternary nanohybrids consisting of conjugated polymers donors and either fullerene or non-fullerene molecular acceptors was prepared and screened for sacrificial photocatalytic hydrogen evolution activity. PCDTBT/PC 60 BM nanohybrid showed a high hydrogen evolution rat...

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Published inChemical communications (Cambridge, England) Vol. 56; no. 5; pp. 679 - 6793
Main Authors Yang, Haofan, Li, Xiaobo, Sprick, Reiner Sebastian, Cooper, Andrew I
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 23.06.2020
Subjects
Donors (electronic)
Fullerenes
Hydrogen evolution
Photocatalysis
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Summary:A library of 237 organic binary/ternary nanohybrids consisting of conjugated polymers donors and either fullerene or non-fullerene molecular acceptors was prepared and screened for sacrificial photocatalytic hydrogen evolution activity. PCDTBT/PC 60 BM nanohybrid showed a high hydrogen evolution rate of 105.2 mmol g −1 h −1 under visible light ( λ > 420 nm). Learning from OPV: Highly efficient nanohybrid photocatalysts that combine conjugated polymer donors with molecular acceptors was discovered for photocatalytic sacrificial hydrogen evolution reaction.
Bibliography:10.1039/d0cc00740d
Electronic supplementary information (ESI) available. See DOI
ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:1359-7345
1364-548X
DOI:10.1039/d0cc00740d