Multi Self-Healable UV Shielding Polyurethane/CeO2 Protective Coating: The Effect of Low-Molecular-Weight Polyols
We prepared a series of polyurethane (PU) coatings with defined contents using poly(tetramethylene oxide)glycol (PTMG) with two different molecular weights (i.e., Mn = 2000 and 650), as well as polydimethyl siloxane (PDMS) with a molecular weight of Mn 550. For every coating, maximum adhesive streng...
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Published in | Polymers Vol. 12; no. 9; p. 1947 |
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Main Authors | , , , , , |
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Language | English |
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Abstract | We prepared a series of polyurethane (PU) coatings with defined contents using poly(tetramethylene oxide)glycol (PTMG) with two different molecular weights (i.e., Mn = 2000 and 650), as well as polydimethyl siloxane (PDMS) with a molecular weight of Mn 550. For every coating, maximum adhesive strength and excellent self-healing character (three times) were found using 6.775 mol% mixed with low-molecular-weight-based polyols (PU-11-3-3). Defined 1.0 wt% CeO2 was also used for the PU-11-3-3 coating (i.e., PU-11-3-3-CeO2) to obtain UV shielding properties. Both the in situ polymerization and blending processes were separately applied during the preparation of the PU-11-3-3-CeO2 coating dispersion. The in situ polymerization-based coating (i.e., PU-11-3-3-CeO2-P) showed similar self-healing properties. The PU-11-3-3-CeO2-P coating also showed excellent UV shielding in real outdoor exposure conditions. |
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AbstractList | We prepared a series of polyurethane (PU) coatings with defined contents using poly(tetramethylene oxide)glycol (PTMG) with two different molecular weights (i.e., Mn = 2000 and 650), as well as polydimethyl siloxane (PDMS) with a molecular weight of Mn 550. For every coating, maximum adhesive strength and excellent self-healing character (three times) were found using 6.775 mol% mixed with low-molecular-weight-based polyols (PU-11-3-3). Defined 1.0 wt% CeO2 was also used for the PU-11-3-3 coating (i.e., PU-11-3-3-CeO2) to obtain UV shielding properties. Both the in situ polymerization and blending processes were separately applied during the preparation of the PU-11-3-3-CeO2 coating dispersion. The in situ polymerization-based coating (i.e., PU-11-3-3-CeO2-P) showed similar self-healing properties. The PU-11-3-3-CeO2-P coating also showed excellent UV shielding in real outdoor exposure conditions. We prepared a series of polyurethane (PU) coatings with defined contents using poly(tetramethylene oxide)glycol (PTMG) with two different molecular weights (i.e., M n = 2000 and 650), as well as polydimethyl siloxane (PDMS) with a molecular weight of M n 550. For every coating, maximum adhesive strength and excellent self-healing character (three times) were found using 6.775 mol% mixed with low-molecular-weight-based polyols (PU-11-3-3). Defined 1.0 wt% CeO 2 was also used for the PU-11-3-3 coating (i.e., PU-11-3-3-CeO 2 ) to obtain UV shielding properties. Both the in situ polymerization and blending processes were separately applied during the preparation of the PU-11-3-3-CeO 2 coating dispersion. The in situ polymerization-based coating (i.e., PU-11-3-3-CeO 2 -P) showed similar self-healing properties. The PU-11-3-3-CeO 2 -P coating also showed excellent UV shielding in real outdoor exposure conditions. |
Author | Rahman, Mohammad Mizanur Kumar, A. Madhan Haq, Md. Bashirul Helal, Aasif Zahir, Md. Hasan Suleiman, Rami |
AuthorAffiliation | 2 Center of Research Excellence in Renewable Energy, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; hzahir@kfupm.edu.sa 4 Department of Petroleum Engineering, College of Petroleum and Geosciences, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia 1 Center of Research Excellence in Corrosion, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; ramismob@kfupm.edu.sa (R.S.); madhankumar@kfupm.edu.sa (A.M.K.) 3 Center of Research Excellence in Nanotechnology, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; aasifh@kfupm.edu.sa |
AuthorAffiliation_xml | – name: 1 Center of Research Excellence in Corrosion, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; ramismob@kfupm.edu.sa (R.S.); madhankumar@kfupm.edu.sa (A.M.K.) – name: 3 Center of Research Excellence in Nanotechnology, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; aasifh@kfupm.edu.sa – name: 4 Department of Petroleum Engineering, College of Petroleum and Geosciences, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia – name: 2 Center of Research Excellence in Renewable Energy, King Fahd University of Petroleum and Minerals, Dhahran 31261, Saudi Arabia; hzahir@kfupm.edu.sa |
Author_xml | – sequence: 1 givenname: Mohammad Mizanur surname: Rahman fullname: Rahman, Mohammad Mizanur – sequence: 2 givenname: Rami orcidid: 0000-0002-6776-9266 surname: Suleiman fullname: Suleiman, Rami – sequence: 3 givenname: Md. Hasan orcidid: 0000-0002-6752-9318 surname: Zahir fullname: Zahir, Md. Hasan – sequence: 4 givenname: Aasif orcidid: 0000-0003-2013-5327 surname: Helal fullname: Helal, Aasif – sequence: 5 givenname: A. Madhan surname: Kumar fullname: Kumar, A. Madhan – sequence: 6 givenname: Md. Bashirul surname: Haq fullname: Haq, Md. Bashirul |
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SubjectTerms | Adhesive strength Adhesives Carbon Cerium oxides coating Coating effects Humidity Metal oxides Molecular weight Nanoparticles Polydimethylsiloxane Polyesters Polymerization Polymers Polyols polyurethane Polyurethane resins Protective coatings Self healing materials self-healing Shielding |
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Title | Multi Self-Healable UV Shielding Polyurethane/CeO2 Protective Coating: The Effect of Low-Molecular-Weight Polyols |
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