Stimuli-responsive tertiary amine methacrylate-based block copolymers: Synthesis, supramolecular self-assembly and functional applications

In the past decade, responsive polymers exhibiting reversible or irreversible changes in physical properties and/or chemical structures in response to external stimuli have been extensively investigated. Among them, tertiary amine methacrylate-based block copolymers represent a unique category consi...

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Bibliographic Details
Published inProgress in polymer science Vol. 39; no. 6; pp. 1096 - 1143
Main Authors Hu, Jinming, Zhang, Guoying, Ge, Zhishen, Liu, Shiyong
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier Ltd 01.06.2014
Elsevier
Subjects
Applied sciences
Exact sciences and technology
Functional applications
Kinetics
Organic polymers
pH-responsive
Physicochemistry of polymers
Polymers with particular properties
Preparation, kinetics, thermodynamics, mechanism and catalysts
Structural fixation
Supramolecular self-assembly
Tertiary amine-based block copolymers
PP
NFHOK
DVS
HEEDTA
MPC
GTP
PS
PMCL
Pt NPs
Supramolecular self-assembly
MEMA
HAuCl4
P3HT
TPFCBPMA
PSSNa
VBA
PTAN
CMA
nBMA
EGDMA
RAFT
PFS
AIE
MAIpGlc
PISA
AD
AzPMA
PUMVS
PGA
Tertiary amine-based block copolymers
THPMA
MW(s)
DPA
PHEGMA
PMEO2MA
Azo
BIEE
cmc
LCST
Kinetics
FOMA
PISR
PDMAEA
PEEP
p-TSCl
UCST
PPO
Au NPs
Functional applications
FITC
tBMA
DHPE
E. coli
HMTETA
PLK1
CEMA
CL
PIC
Structural fixation
2VP
HEMA
EBiB
pH-responsive
AmB
GPC
PAM
PEGMA
PMAGIc
NaBH4
AzoMA
(P)QA
NIPAM
PAEMA
MTS
PTMS
(M)AA
ImPAA
DHBC(s)
CuBr
MAPTAC
TBABB
ATRP
EEP
ROP
cryo-TEM
pDNA
IEP
PMPDSAH
DLA
M(M)A
CuCl
Ea
HPMA
PDMS
LLA
CRP
BPN
QDs
Mn
QDMA
AzoM
PBLG
POEGMA
DLS
PMDETA
GAMA
PSVBP
TDA
DP(s)
PDF
PAPMA
Nagg
NHS
DMA
ARGET
DEA
PFOMA
VEGF
Con A
LAMA
bpy
siRNA
CCL
PGMA
PSoMA
PDHMA
SAXS
PB
β-CD
PEG
PF
PI
SCL
DTBP
PET
Review
Mechanism
Monodispersed polymer
Preparation
Molecular aggregation
Methacrylate copolymer
Aqueous solution
Amine copolymer
Medical application
Block copolymer
Amphiphilic polymer
Online AccessGet full text

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Abstract In the past decade, responsive polymers exhibiting reversible or irreversible changes in physical properties and/or chemical structures in response to external stimuli have been extensively investigated. Among them, tertiary amine methacrylate-based block copolymers represent a unique category considering their responsiveness to multiple external stimuli (e.g., pH, temperature and salts), which are essentially relevant to the biological milieu. These intriguing properties allow for their applications in a variety of fields ranging from drug or gene delivery, imaging, diagnostics, antibacterial coatings, catalysis, and bio-separations. This review article highlights tertiary amine methacrylate-based block copolymers, focusing on recent advances in the synthesis of tertiary amine methacrylate-based block copolymers with varying chemical structures and chain topologies, their supramolecular self-assembly in aqueous media as well as in the bulk state, and the emerging functional applications.
AbstractList In the past decade, responsive polymers exhibiting reversible or irreversible changes in physical properties and/or chemical structures in response to external stimuli have been extensively investigated. Among them, tertiary amine methacrylate-based block copolymers represent a unique category considering their responsiveness to multiple external stimuli (e.g., pH, temperature and salts), which are essentially relevant to the biological milieu. These intriguing properties allow for their applications in a variety of fields ranging from drug or gene delivery, imaging, diagnostics, antibacterial coatings, catalysis, and bio-separations. This review article highlights tertiary amine methacrylate-based block copolymers, focusing on recent advances in the synthesis of tertiary amine methacrylate-based block copolymers with varying chemical structures and chain topologies, their supramolecular self-assembly in aqueous media as well as in the bulk state, and the emerging functional applications.
Author Ge, Zhishen
Zhang, Guoying
Hu, Jinming
Liu, Shiyong
Author_xml – sequence: 1
  givenname: Jinming
  surname: Hu
  fullname: Hu, Jinming
– sequence: 2
  givenname: Guoying
  surname: Zhang
  fullname: Zhang, Guoying
– sequence: 3
  givenname: Zhishen
  surname: Ge
  fullname: Ge, Zhishen
– sequence: 4
  givenname: Shiyong
  surname: Liu
  fullname: Liu, Shiyong
  email: sliu@ustc.edu.cn
BackLink http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28512799$$DView record in Pascal Francis
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Issue 6
Keywords PP
NFHOK
DVS
HEEDTA
MPC
GTP
PS
PMCL
Pt NPs
Supramolecular self-assembly
MEMA
HAuCl4
P3HT
TPFCBPMA
PSSNa
VBA
PTAN
CMA
nBMA
EGDMA
RAFT
PFS
AIE
MAIpGlc
PISA
AD
AzPMA
PUMVS
PGA
Tertiary amine-based block copolymers
THPMA
MW(s)
DPA
PHEGMA
PMEO2MA
Azo
BIEE
cmc
LCST
Kinetics
FOMA
PISR
PDMAEA
PEEP
p-TSCl
UCST
PPO
Au NPs
Functional applications
FITC
tBMA
DHPE
E. coli
HMTETA
PLK1
CEMA
CL
PIC
Structural fixation
2VP
HEMA
EBiB
pH-responsive
AmB
GPC
PAM
PEGMA
PMAGIc
NaBH4
AzoMA
(P)QA
NIPAM
PAEMA
MTS
PTMS
(M)AA
ImPAA
DHBC(s)
CuBr
MAPTAC
TBABB
ATRP
EEP
ROP
cryo-TEM
pDNA
IEP
PMPDSAH
DLA
M(M)A
CuCl
Ea
HPMA
PDMS
LLA
CRP
BPN
QDs
Mn
QDMA
AzoM
PBLG
POEGMA
DLS
PMDETA
GAMA
PSVBP
TDA
DP(s)
PDF
PAPMA
Nagg
NHS
DMA
ARGET
DEA
PFOMA
VEGF
Con A
LAMA
bpy
siRNA
CCL
PGMA
PSoMA
PDHMA
SAXS
PB
β-CD
PEG
PF
PI
SCL
DTBP
PET
Review
Mechanism
Monodispersed polymer
Preparation
Molecular aggregation
Methacrylate copolymer
Aqueous solution
Amine copolymer
Medical application
Block copolymer
Amphiphilic polymer
Language English
License CC BY 4.0
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Snippet In the past decade, responsive polymers exhibiting reversible or irreversible changes in physical properties and/or chemical structures in response to external...
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elsevier
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SubjectTerms Applied sciences
Exact sciences and technology
Functional applications
Kinetics
Organic polymers
pH-responsive
Physicochemistry of polymers
Polymers with particular properties
Preparation, kinetics, thermodynamics, mechanism and catalysts
Structural fixation
Supramolecular self-assembly
Tertiary amine-based block copolymers
Title Stimuli-responsive tertiary amine methacrylate-based block copolymers: Synthesis, supramolecular self-assembly and functional applications
URI https://dx.doi.org/10.1016/j.progpolymsci.2013.10.006
Volume 39
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