A microcavity-controlled, current-driven, on-chip nanotube emitter at infrared wavelengths

• Published in: Nature nanotechnology Vol. 3; no. 10; pp. 609 - 613
• Main Authors: Xia, Fengnian, Avouris, Phaedon, Steiner, Mathias, Lin, Yu-ming
• Format: Journal Article
• Language: English
• Published: London Nature Publishing Group UK 01.10.2008; Nature Publishing Group
• Subjects: Carbon; Chemistry and Materials Science; Electrochemistry - instrumentation; Electrochemistry - methods; Electrons; Emissions; Infrared Rays; Injection; letter; Luminescence; Materials Science; Materials Testing - methods; Microscopy, Electron, Scanning; Nanotechnology; Nanotechnology - instrumentation; Nanotechnology - methods; Nanotechnology and Microengineering; Nanotubes, Carbon - chemistry; Optical properties; Optics and Photonics - instrumentation; Optics and Photonics - methods; Polymethyl methacrylate; Resonance; Semiconductors; Spectrum Analysis, Raman; Transistors; Wavelengths
• ISSN: 1748-3387; 1748-3395
• DOI: 10.1038/nnano.2008.241

Recent studies of the optical properties of semiconducting single-walled carbon nanotubes 1 , 2 , 3 , 4 , 5 , 6 suggest that these truly nanometre-scale systems have a promising future in nanophotonics, in addition to their well-known potential in electronics 7 , 8 . Semiconducting single-walled nanotubes have a direct, diameter-dependent bandgap 8 and can be excited readily by current injection, which makes them attractive as nano-emitters. The electroluminescence is spectrally broad, spatially non-directional, and the radiative yield is low 5 , 9 . Here we report the monolithic integration of a single, electrically excited, semiconducting nanotube transistor with a planar λ/2 microcavity 10 , 11 , 12 , 13 , thus taking an important first step in the development of nanotube-based nanophotonic devices. The spectral full-width at half-maximum of the emission is reduced from ∼300 to ∼40 nm at a cavity resonance of 1.75 µm, and the emission becomes highly directional. The maximum enhancement of the radiative rate is estimated to be 4. We also show that both the optically and electrically excited luminescence of single-walled nanotubes involve the same E 11 excitonic transition. Semiconducting carbon nanotubes have a direct bandgap, which means that they could form the basis of nanoscale light sources. However, nanotubes tend to emit light over a broad range of wavelengths and directions. Placing the nanotube in a microcavity reduces the spectral width of the output and makes the emission highly directional. This microcavity-controlled, current-driven on-chip emitter is thus an important first step in the development of nanotube-based nanophotonic devices.