Opacity effects on soft X-ray spectra from highly charged lanthanide ions in laser-produced plasmas

• Published in: Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms Vol. 408; pp. 253 - 256
• Main Authors: Suzuki, C., Higashiguchi, T., Sasanuma, A., Arai, G., Fujii, Y., Kondo, Y., Dinh, T.-H., Koike, F., Murakami, I., O’Sullivan, G.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 01.10.2017
• Subjects: Lanthanide ions; Laser-produced plasmas; Opacity; Soft X-ray spectra; Soft X-ray spectra; Laser-produced plasmas; Opacity; Lanthanide ions
• ISSN: 0168-583X; 1872-9584
• DOI: 10.1016/j.nimb.2017.03.094

We have observed soft X-ray spectra from highly charged ions of seven different lanthanide elements with atomic numbers ranging from 60 to 70 in laser-produced plasmas (LPPs) using CO2 and Nd:YAG laser systems, the wavelengths of which are 10.6μm and 1.064μm, respectively. The spectral feature drastically changes between the two types of LPPs due primarily to the difference in opacity. Narrowband quasicontinuum features arising from n=4–4 transitions, the centre wavelength of which systematically moves to shorter wavelength as the atomic number (Z) increases, are observed in the CO2 LPPs, accompanied by sharp peaks coinciding with the strongest resonance lines of Pd-like ions for lower Z elements. In contrast, the quasicontinuum bands are broader and smoother in the Nd:YAG LPPs, appearing with bands of n=4–5 transitions on the shorter wavelength side. The results are also discussed based on comparisons with atomic structure calculations for ions with outermost 4d and 4f subshells.