Experimental investigation of hydrate accumulation distribution in gas seeping system using a large scale three-dimensional simulation device

• Published in: Chemical engineering science Vol. 82; pp. 246 - 259
• Main Authors: Su, Ke-Hua, Sun, Chang-Yu, Dandekar, Abhijit, Liu, Bei, Sun, Wei-Zhi, Cao, Meng-Chang, Li, Nan, Zhong, Xiao-Yu, Guo, Xu-Qiang, Ma, Qing-Lan, Yang, Lan-Ying, Chen, Guang-Jin
• Format: Journal Article
• Language: English
• Published: Kidlington Elsevier Ltd 12.09.2012; Elsevier
• Subjects: Accumulation; acoustics; Applied sciences; cement; Chemical engineering; electrical resistance; Exact sciences and technology; Gases; Hydrate; Hydrodynamics of contact apparatus; Kinetics; methane; natural gas; Porous media; sediments; Simulation; thermal properties; Porous media; Gases; Hydrate; Kinetics; Simulation; Accumulation; Saturation; Porous medium; Sediments; Real time; Flow field; Real time system; Aggregation; Design; Thermal properties; Three dimensional model; Cement; Production; Gas hydrates; Natural gas
• ISSN: 0009-2509; 1873-4405
• DOI: 10.1016/j.ces.2012.07.029

A novel three-dimensional natural gas hydrate physical simulation device, with a capacity of 0.196m3 and maximum operating pressure of 32MPa, was designed and developed to study the accumulation and exploitation of hydrate-bearing sediment in the natural environment. Acoustic, electrical, and thermal properties at different positions can be collected in real-time to analyze the evolution of hydrate-bearing porous media during the accumulation of hydrate or the production of natural gas. A preliminary experiment was performed to investigate the behaviors of hydrate formation and aggregation in sediment in conditions simulating a gas seeping system. The experimental results showed the methane seeping route has a critical effect on hydrate formation and accumulation within the sediment, and the location of hydrate-rich region. The distribution of hydrate in sediment was controlled by fluid flow field, which was also proven by the simulation of FLUENTTM code. A modified form of Archie’s law was used to correlate hydrate saturation with the electrical resistivity data. The process of hydrate growth, that hydrate first cement and bridge grains, is also deduced from the acoustic velocity data. ► A novel three-dimensional natural gas hydrate physical simulation device is built. ► Hydrate formation and accumulation for gas seeping system is simulated. ► Hydrate growth in sediment is detected by thermal, electrical, and acoustic sensors. ► Methane seeping route and fluid flow field affect on hydrate accumulation.