Experiments with a prototype titanium hot cavity surface ionization source intended for electromagnetic separation of radioactive samarium and other lanthanide elements

• Published in: Applied radiation and isotopes Vol. 170; p. 109621
• Main Authors: Jeffries, Brad D., O'Donnell, Valentina, Norgard, Peter, Robertson, J. David, Higgins, Barry, Gahl, John
• Format: Journal Article
• Language: English
• Published: England Elsevier Ltd 01.04.2021; Elsevier
• Subjects: 07 ISOTOPE AND RADIATION SOURCES; 153Sm (samarium-153); Electromagnetic isotope separator; Medical radioisotopes; Surface ionization source; Surface ionization source; Medical radioisotopes; Electromagnetic isotope separator; 153Sm (samarium-153); Sm (samarium-153)
• ISSN: 0969-8043; 1872-9800
• DOI: 10.1016/j.apradiso.2021.109621

This paper reports experimental results of a prototype titanium surface ionization source. For the first time, a lanthanide ion beam has been produced with a surface ionizer composed completely of titanium metal. Titanium does not readily activate with neutron irradiation. This offers the potential for inserting an ion source made of titanium directly into a reactor with a pre-loaded non-radioactive lanthanide target. This seamlessly integrates target irradiation with isotope separation, eliminating post irradiation sample manipulation. Samarium ion beam currents up to 960 nA have been produced in an off-line test bench equipped with rudimentary beam optics. This is a crucial step toward the development of an ionization source adopted for the electromagnetic isotope separator (EMIS) facility, which has been designed for high throughput separations of radioactive 153Sm and other lanthanides of interest in the field of nuclear medicine. The ion current and important factors affecting the performance of the ion source, such as the ionizer temperature and thermal gradient, are discussed. The experimental results are presented together with a discussion of future modifications to optimize the overall surface ionization source performance. •Surface ionization source designed for electromagnetic isotope separation of lanthanides.•A samarium ion beam has been produced with a hot surface ionizer composed completely of titanium metal.•The temporal development of the samarium ion current and temperature of the prototype surface ion source is presented.