Recent progress in the development of anodes for asymmetric supercapacitors

Asymmetric supercapacitors (ASCs) have great promise as an alternative power source in portable electronics and hybrid vehicles. To date, the imbalance between the developments of anode and cathode materials for ASCs remains a crucial issue, which makes the development of high-performance anodes a s...

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Published inJournal of materials chemistry. A, Materials for energy and sustainability Vol. 4; no. 13; pp. 4634 - 4658
Main Authors Yu, Minghao, Wang, Zilong, Han, Yi, Tong, Yexiang, Lu, Xihong, Yang, Shihe
Format Journal Article
LanguageEnglish
Published 01.01.2016
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Summary:Asymmetric supercapacitors (ASCs) have great promise as an alternative power source in portable electronics and hybrid vehicles. To date, the imbalance between the developments of anode and cathode materials for ASCs remains a crucial issue, which makes the development of high-performance anodes a significant research direction. In this article, we review recent achievements in the design and fabrication of novel ASC anodes, which fall into the categories of carbon based, metal oxides based, metal nitrides based, and other anodes. The merits and demerits of these anodes are analyzed and discussed based on the results published in the literature in the past few years. The strategies employed to overcome the specific drawbacks of various anode materials are elaborated. Moreover, the electrochemical performances of ASC devices assembled with these anodes are critically examined and compared. Finally, we further project the trends and challenges in the future development of high-performance ASC anodes. Recent advances and challenges in anodes for asymmetric supercapacitors are reviewed and discussed.
Bibliography:Minghao Yu received his B.S. degree in polymer chemistry from SunYat-Sen University in 2012. He is currently a 4
Zilong Wang received his B.S. (2010) and M.S. (2012) in the School of Chemistry and Chemical Engineering from SunYat-Sen University in China. He is currently a Ph.D. candidate in Prof. Shihe Yang's group in the Department of Chemistry of the Hong Kong University of Science and Technology. His current research focuses on nanomaterials and their applications for energy storage and fuel cells.
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Shihe Yang received his B.S. (1982) in Chemistry from SunYat-Sen University in China. Through the US-China CGP program, he was admitted to Rice University in 1983 and obtained a Ph.D. in Physical Chemistry in 1988 (with Prof. Richard E. Smalley). He did his post-doctoral research at Argonne National Laboratory and the University of Toronto (with Prof. John C. Polanyi) before joining the faculty at the Hong Kong University of Science and Technology in 1992, where he is currently a full Professor. His current research interest is focused on energy conversion science by drawing on the understanding, manipulation and applications of low-dimensional nanosystems, materials and interfaces.
year Ph.D. student of materials physics and chemistry in Prof. Yexiang Tong's group at SunYat-Sen University. His research focuses on the development of nanostructured materials for application in supercapacitors.
Prof. Xihong Lu received his B.S. degree in Applied Chemistry from SunYat-Sen University in 2008, and then obtained his Ph.D. in Physical Chemistry from SunYat-Sen University in 2013. He is now an associate professor in the School of Chemistry and Chemical Engineering at SunYat-Sen University. His current research focuses on the design and synthesis of functionally nanostructured materials for applications in energy conversion and storage, such as photoelectrochemical/photocatalytic water splitting, supercapacitors and Li ion batteries.
Yi Han is currently an undergraduate student in the School of Chemistry and Chemical Engineering at SunYat-Sen University. He joined Prof. Lu's group in 2013. His current research focuses on the design of metal oxide/nitride nanomaterials and their application in energy storage.
Prof. Yexiang Tong received his B.S. in General Chemistry in 1985, M.S. in Physical Chemistry in 1988, and Ph.D. in Organic Chemistry in 1999 from SunYat-Sen University. He joined SunYat-Sen University as an assistant professor of chemistry (1988), and later became an associate professor (1995) and professor (2001). His current research focuses on the electrochemical synthesis of alloys, intermetallic compounds and metal oxide nanomaterials, and investigation of their applications for energy conversion and storage.
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ISSN:2050-7488
2050-7496
DOI:10.1039/c5ta10542k