Mechanical Resonant Sensing of Spin Texture Dynamics in a 2D Antiferromagnet

• Published in: Advanced materials (Weinheim) Vol. 37; no. 29; pp. e2420168 - n/a
• Main Authors: Yousuf, S M Enamul Hoque, Wang, Yunong, Ramachandran, Shreyas, Koptur‐Palenchar, John, Tarantini, Chiara, Xiang, Li, McGill, Stephen, Smirnov, Dmitry, Santos, Elton J. G., Feng, Philip X.‐L., Zhang, Xiao‐Xiao
• Format: Journal Article
• Language: English
• Published: Germany Wiley Subscription Services, Inc 01.07.2025; John Wiley and Sons Inc
• Subjects: 2D materials; Actuation; Antiferromagnetism; Coupling; Data processing; Domain walls; Hypothetical particles; magnetic properties; Magnetic structure; Magnetic transitions; Magnetostriction; NEMS; Particle theory; Resonant frequencies; Shearing; Spin dynamics; spintronics; Strain; Texture; spintronics; NEMS; magnetic properties; 2D materials
• ISSN: 0935-9648; 1521-4095; 1521-4095
• DOI: 10.1002/adma.202420168

The coupling between the spin degrees of freedom and macroscopic mechanical motions, including striction, shearing, and rotation, has attracted wide interest with applications in actuation, transduction, and information processing. Experiments so far have established the mechanical responses to the long‐range ordered or isolated single spin states. However, it remains elusive whether mechanical motions can couple to a different type of magnetic structure, the non‐collinear spin textures, which exhibit nanoscale spatial variations of spin (domain walls, skyrmions, etc.) and are promising candidates to realize high‐speed computing devices. Here, collective spin texture dynamics is detected with nanoelectromechanical resonators fabricated from 2D antiferromagnetic (AFM) MnPS3 with 10−9 strain sensitivity. By examining radio frequency mechanical oscillations under magnetic fields, new magnetic transitions are identified with sharp dips in resonant frequency. They are attributed to collective AFM domain wall motions as supported by the analytical modeling of magnetostriction and large‐scale spin‐dynamics simulations. Additionally, an abnormally large modulation in the mechanical nonlinearity at the transition field infers a fluid‐like response due to ultrafast domain motion. The work establishes a strong coupling between spin texture and mechanical dynamics, laying the foundation for electromechanical manipulation of spin texture and developing quantum hybrid devices. Detection of antiferromagnetic spin texture in a 2D magnetic crystal is achieved through nanomechanical resonators at radio frequencies. Sharp magnetic transitions that lead to abrupt changes in mechanical linear and nonlinear responses are assigned to antiferromagnetic domain motions. The results indicate rich and fluid‐like dynamics between the coupled spin and lattice at the transition field.