Brightening of dark excitons in monolayers of semiconducting transition metal dichalcogenides

We present low-temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field B applied to monolayers of different semiconducting transition metal dichalcogenides. For WSe2 and WS2 monolayers, the dark exciton emission is observed a...

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Published in2d materials Vol. 4; no. 2; pp. 21003 - 21008
Main Authors Molas, M R, Faugeras, C, Slobodeniuk, A O, Nogajewski, K, Bartos, M, Basko, D M, Potemski, M
Format Journal Article
LanguageEnglish
Published IOP Publishing 01.06.2017
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Abstract We present low-temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field B applied to monolayers of different semiconducting transition metal dichalcogenides. For WSe2 and WS2 monolayers, the dark exciton emission is observed at   50 meV below the bright exciton peak and displays a characteristic doublet structure whose intensity grows with B2, while no magnetic field induced emission peaks appear for MoSe2 monolayer. Our experiments also show that the MoS2 monolayer has a dark exciton ground state with a dark-bright exciton splitting energy of   100 meV.
AbstractList We present low-temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field B applied to monolayers of different semiconducting transition metal dichalcogenides. For WSe2 and WS2 monolayers, the dark exciton emission is observed at   50 meV below the bright exciton peak and displays a characteristic doublet structure whose intensity grows with B2, while no magnetic field induced emission peaks appear for MoSe2 monolayer. Our experiments also show that the MoS2 monolayer has a dark exciton ground state with a dark-bright exciton splitting energy of   100 meV.
Author Basko, D M
Slobodeniuk, A O
Bartos, M
Potemski, M
Faugeras, C
Molas, M R
Nogajewski, K
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  givenname: M R
  surname: Molas
  fullname: Molas, M R
  email: maciej.molas@gmail.com
  organization: CNRS-UGA-UPS-INSA-EMFL Laboratoire National des Champs Magnétiques Intenses, 25, avenue des Martyrs, 38042 Grenoble, France
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  surname: Faugeras
  fullname: Faugeras, C
  organization: CNRS-UGA-UPS-INSA-EMFL Laboratoire National des Champs Magnétiques Intenses, 25, avenue des Martyrs, 38042 Grenoble, France
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  givenname: A O
  surname: Slobodeniuk
  fullname: Slobodeniuk, A O
  organization: CNRS-UGA-UPS-INSA-EMFL Laboratoire National des Champs Magnétiques Intenses, 25, avenue des Martyrs, 38042 Grenoble, France
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  givenname: K
  surname: Nogajewski
  fullname: Nogajewski, K
  organization: CNRS-UGA-UPS-INSA-EMFL Laboratoire National des Champs Magnétiques Intenses, 25, avenue des Martyrs, 38042 Grenoble, France
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  surname: Bartos
  fullname: Bartos, M
  organization: Brno University of Technology CEITEC BUT, Purkynova 123,61200 Brno, Czech Republic
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  surname: Basko
  fullname: Basko, D M
  organization: Université de Grenoble-Alpes and CNRS Laboratoire de Physique et Modélisation des Milieux Condensés, 25 rue des Martyrs, 38042 Grenoble, France
– sequence: 7
  givenname: M
  surname: Potemski
  fullname: Potemski, M
  email: marek.potemski@lncmi.cnrs.fr
  organization: CNRS-UGA-UPS-INSA-EMFL Laboratoire National des Champs Magnétiques Intenses, 25, avenue des Martyrs, 38042 Grenoble, France
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Snippet We present low-temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field B applied to...
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SubjectTerms Condensed Matter
dark excitons
Disordered Systems and Neural Networks
Materials Science
molybdenum diselenide
molybdenum disulfide
Physics
Quantum Physics
transition metal dichalcogenides monolayers
tungsten diselenide
tungsten disulfide
Voigt configuration
Title Brightening of dark excitons in monolayers of semiconducting transition metal dichalcogenides
URI https://iopscience.iop.org/article/10.1088/2053-1583/aa5521
https://hal.science/hal-01992291
Volume 4
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