Rh-Catalyzed oxidative C–H activation/annulation: converting anilines to indoles using molecular oxygen as the sole oxidant

A practical and efficient Rh( iii )-catalyzed aerobic C–H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.

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Bibliographic Details
Published inChemical communications (Cambridge, England) Vol. 50; no. 33; pp. 4331 - 4334
Main Authors Zhang, Guoying, Yu, Hui, Qin, Guiping, Huang, Hanmin
Format Journal Article
LanguageEnglish
Published CAMBRIDGE Royal Soc Chemistry 01.01.2014
Subjects
Activation
Alkynes
Aniline
carbon-hydrogen bond activation
catalytic activity
chemical reactions
Chemistry
Chemistry, Multidisciplinary
Indoles
Oxidants
Oxidizing agents
Oxygen
Physical Sciences
rhodium
Science & Technology
Sole
FUNCTIONALIZATION
HAPALINDOLES
ACETANILIDES
ACTIVATION
AMINATION
ANNULATION
EFFICIENT SYNTHESIS
POTASSIUM
BOND
CYCLIZATION
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Abstract A practical and efficient Rh( iii )-catalyzed aerobic C–H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.
AbstractList A practical and efficient Rh(III)-catalyzed aerobic C-H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.
A practical and efficient Rh(III)-catalyzed aerobic C-H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.A practical and efficient Rh(III)-catalyzed aerobic C-H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.
A practical and efficient Rh( iii )-catalyzed aerobic C–H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines and alkynes. The protocol could be conducted under mild conditions and used environmentally friendly oxygen as the sole clear oxidant.
Author Yu, Hui
Zhang, Guoying
Huang, Hanmin
Qin, Guiping
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  givenname: Guoying
  surname: Zhang
  fullname: Zhang, Guoying
  organization: State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, China
– sequence: 2
  givenname: Hui
  surname: Yu
  fullname: Yu, Hui
  organization: State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, China
– sequence: 3
  givenname: Guiping
  surname: Qin
  fullname: Qin, Guiping
  organization: State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, China
– sequence: 4
  givenname: Hanmin
  surname: Huang
  fullname: Huang, Hanmin
  organization: State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou, China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/24643726$$D View this record in MEDLINE/PubMed
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Issue 33
Keywords FUNCTIONALIZATION
HAPALINDOLES
ACETANILIDES
ACTIVATION
AMINATION
ANNULATION
EFFICIENT SYNTHESIS
POTASSIUM
BOND
CYCLIZATION
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Snippet A practical and efficient Rh( iii )-catalyzed aerobic C–H activation has been developed for the facile synthesis of a broad range of indoles from simple...
A practical and efficient Rh(III)-catalyzed aerobic C-H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines...
A practical and efficient Rh(iii)-catalyzed aerobic C-H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines...
A practical and efficient Rh(iii)-catalyzed aerobic C–H activation has been developed for the facile synthesis of a broad range of indoles from simple anilines...
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SubjectTerms Activation
Alkynes
Aniline
carbon-hydrogen bond activation
catalytic activity
chemical reactions
Chemistry
Chemistry, Multidisciplinary
Indoles
Oxidants
Oxidizing agents
Oxygen
Physical Sciences
rhodium
Science & Technology
Sole
Title Rh-Catalyzed oxidative C–H activation/annulation: converting anilines to indoles using molecular oxygen as the sole oxidant
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https://www.ncbi.nlm.nih.gov/pubmed/24643726
https://www.proquest.com/docview/1511390794
https://www.proquest.com/docview/1893880580
https://www.proquest.com/docview/2335127892
Volume 50
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