Hydrogen‐Bonded Organic Framework for High‐Performance Lithium/Sodium‐Iodine Organic Batteries
The rechargeable lithium/sodium‐iodine battery (Li/Na‐I2) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded organic framework (HOF) linked to the Ti3C2Tx MXene complex (HOF@Ti3C2Tx) has been presented for iodine loading. HOF is self‐assembled by organ...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 48; pp. e202213276 - n/a |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
25.11.2022
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The rechargeable lithium/sodium‐iodine battery (Li/Na‐I2) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded organic framework (HOF) linked to the Ti3C2Tx MXene complex (HOF@Ti3C2Tx) has been presented for iodine loading. HOF is self‐assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I2‐based batteries. The I2/HOF@Ti3C2Tx exhibits large reversible capacities of 260.2 and 207.6 mAh g−1 at 0.2 C after repeated cycling for Li‐I2 and Na‐I2 batteries, respectively. This work can gain insights into the HOF‐related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions.
A complex of a hydrogen‐bonded organic framework (HOF) linked with Ti3C2Tx MXene was designed and adopted as electrodes with excellent cyclic stability and rate‐performances in Li‐I2 and Na‐I2 batteries. |
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| AbstractList | The rechargeable lithium/sodium-iodine battery (Li/Na-I2 ) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen-bonded organic framework (HOF) linked to the Ti3 C2 Tx MXene complex (HOF@Ti3 C2 Tx ) has been presented for iodine loading. HOF is self-assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I2 -based batteries. The I2 /HOF@Ti3 C2 Tx exhibits large reversible capacities of 260.2 and 207.6 mAh g-1 at 0.2 C after repeated cycling for Li-I2 and Na-I2 batteries, respectively. This work can gain insights into the HOF-related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions.The rechargeable lithium/sodium-iodine battery (Li/Na-I2 ) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen-bonded organic framework (HOF) linked to the Ti3 C2 Tx MXene complex (HOF@Ti3 C2 Tx ) has been presented for iodine loading. HOF is self-assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I2 -based batteries. The I2 /HOF@Ti3 C2 Tx exhibits large reversible capacities of 260.2 and 207.6 mAh g-1 at 0.2 C after repeated cycling for Li-I2 and Na-I2 batteries, respectively. This work can gain insights into the HOF-related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions. The rechargeable lithium/sodium‐iodine battery (Li/Na‐I 2 ) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded organic framework (HOF) linked to the Ti 3 C 2 T x MXene complex (HOF@Ti 3 C 2 T x ) has been presented for iodine loading. HOF is self‐assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I 2 ‐based batteries. The I 2 /HOF@Ti 3 C 2 T x exhibits large reversible capacities of 260.2 and 207.6 mAh g −1 at 0.2 C after repeated cycling for Li‐I 2 and Na‐I 2 batteries, respectively. This work can gain insights into the HOF‐related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions. The rechargeable lithium/sodium‐iodine battery (Li/Na‐I2) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded organic framework (HOF) linked to the Ti3C2Tx MXene complex (HOF@Ti3C2Tx) has been presented for iodine loading. HOF is self‐assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I2‐based batteries. The I2/HOF@Ti3C2Tx exhibits large reversible capacities of 260.2 and 207.6 mAh g−1 at 0.2 C after repeated cycling for Li‐I2 and Na‐I2 batteries, respectively. This work can gain insights into the HOF‐related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions. The rechargeable lithium/sodium‐iodine battery (Li/Na‐I2) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded organic framework (HOF) linked to the Ti3C2Tx MXene complex (HOF@Ti3C2Tx) has been presented for iodine loading. HOF is self‐assembled by organic monomers through hydrogen bonding interactions between each monomer. It leads to numerous cavities in HOF structure, which can encapsulate iodine through various adsorptive sites and intermolecular interactions. The unique structure of complex can accelerate the nucleation of iodine, achieve fast reaction kinetics, stabilize iodide and retard the shuttle effect, thus improving the cycling stability of I2‐based batteries. The I2/HOF@Ti3C2Tx exhibits large reversible capacities of 260.2 and 207.6 mAh g−1 at 0.2 C after repeated cycling for Li‐I2 and Na‐I2 batteries, respectively. This work can gain insights into the HOF‐related energy storage application with reversible iodine encapsulation and its related redox reaction mechanisms with Li and Na metal ions. A complex of a hydrogen‐bonded organic framework (HOF) linked with Ti3C2Tx MXene was designed and adopted as electrodes with excellent cyclic stability and rate‐performances in Li‐I2 and Na‐I2 batteries. |
| Author | Cao, Yingnan Zhang, Yifan Guo, Chaofei Wang, Yong Han, Bo Sun, Weiwei |
| Author_xml | – sequence: 1 givenname: Chaofei surname: Guo fullname: Guo, Chaofei organization: Shanghai University – sequence: 2 givenname: Bo surname: Han fullname: Han, Bo organization: Central South University – sequence: 3 givenname: Weiwei orcidid: 0000-0003-3949-6026 surname: Sun fullname: Sun, Weiwei organization: Shanghai University – sequence: 4 givenname: Yingnan surname: Cao fullname: Cao, Yingnan organization: Shanghai University – sequence: 5 givenname: Yifan surname: Zhang fullname: Zhang, Yifan organization: Shanghai University – sequence: 6 givenname: Yong orcidid: 0000-0003-3489-7672 surname: Wang fullname: Wang, Yong email: yongwang@shu.edu.cn organization: Shanghai University |
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| Snippet | The rechargeable lithium/sodium‐iodine battery (Li/Na‐I2) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded... The rechargeable lithium/sodium‐iodine battery (Li/Na‐I 2 ) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen‐bonded... The rechargeable lithium/sodium-iodine battery (Li/Na-I2 ) is a promising candidate for meeting the growing energy demand. Herein, a flexible hydrogen-bonded... |
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| SubjectTerms | Adsorptivity Cycles Encapsulation Energy demand Energy storage Hydrogen Hydrogen bonding Hydrogen-Bonded Organic Framework Iodides Iodine Lithium Lithium/Sodium-Iodine Organic Batteries Metal ions Monomers Nucleation Reaction kinetics Reaction mechanisms Rechargeable batteries Redox Reaction Redox reactions Sodium Ti3C2Tx MXene |
| Title | Hydrogen‐Bonded Organic Framework for High‐Performance Lithium/Sodium‐Iodine Organic Batteries |
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