Experimental characterization of three-dimensional Graphene’s thermoacoustic response and its theoretical modelling

• Published in: Carbon (New York) Vol. 169; pp. 382 - 394
• Main Authors: Ngoh, Zhi Lin, Guiraud, Pierre, Tan, Dunlin, Giordano, Stefano, Bou-Matar, Olivier, Teo, Edwin Hang Tong, Pernod, Philippe, Coquet, Philippe, Lardat, Raphael
• Format: Journal Article
• Language: English
• Published: New York Elsevier Ltd 01.11.2020; Elsevier BV; Elsevier
• Subjects: Acoustics; Carbon; Chemical synthesis; Chemical vapor deposition; Engineering Sciences; Graphene; Loudspeaker; Materials; Microstructure; Nanostructure; Nanostructured materials; Raman spectroscopy; Simulation; Temperature; Theoretical modelling; Thermoacoustics; Three dimensional models; Three-dimensional graphene (3D-C); Theoretical modelling; Thermoacoustics; Three-dimensional graphene (3D-C); Loudspeaker; Chemical vapor deposition; theoretical modelling; three-dimensional graphene (3D-C); loudspeaker; chemical vapor deposition; thermoacoustics
• ISSN: 0008-6223; 1873-3891
• DOI: 10.1016/j.carbon.2020.06.045

In the past decade, a lot of research has been conducted on the potential of carbon nanostructured materials to emit sound via thermoacoustics through both simulations and experiments. However, experimental validation of simulations for three-dimensional graphene (3D-C), which has a complicated 3D structure, has yet to be achieved. In this paper, 3D-C is synthesized via thermal chemical vapor deposition and its microstructure and quality tested using Scanning Electron Microscopy and Raman spectroscopy respectively. Then, a two temperature model is used to predict the effects of numerous parameters: frequency, input power, sample size, connection area, connection path, pores per inch, thickness, compression as well as the addition of a backing on the acoustic performance and temperature of the sample. The experimental results presented in this paper validate the predictions of the adopted two temperature model. The efficiency of 3D-C is then compared with results presented in other studies to understand how the presented 3D-C fared against ones from the literature as well as other carbon nanostructured materials. [Display omitted]