3D analysis of TRISO fuel compacts via X-ray computed tomography

• Published in: Journal of nuclear materials Vol. 565; no. C; p. 153745
• Main Authors: Kane, Joshua J., Marshall, Douglas W., Cordes, Nikolaus L., Chuirazzi, William C., Kombaiah, Boopathy, van Rooyen, Isabella, Stempien, John D.
• Format: Journal Article
• Language: English
• Published: Amsterdam Elsevier B.V 01.07.2022; Elsevier BV; Elsevier
• Subjects: 3D image processing; Binding energy; Compacts; Computed tomography; Coordination numbers; Fractions; Image analysis; Image processing; Kernels; Nondestructive analysis; Oxycarbides; Packing; Porosity; Spatial distribution; Tomography; TRISO fuel; TRISO particles; Uranium; X-ray computed tomography; 3D image processing; X-ray computed tomography; TRISO particles; Nondestructive analysis; TRISO fuel
• ISSN: 0022-3115; 1873-4820
• DOI: 10.1016/j.jnucmat.2022.153745

Low-enriched uranium oxycarbide (LEUCO) and surrogate tristructural isotropic (TRISO)- coated-particle compacts with particle volumetric packing fractions of 25%, 40%, and 48% were imaged utilizing X-ray-computed tomography. Subsequent 3D image analysis identified and further quantified kernel size, sphericity, and observed porosity. In addition, the spatial distribution, coordination number, and kernel-nearest neighbors were analyzed and compared for the different packing fractions. Metrics such as observed porosity and sphericity enabled quantification and screening for abnormal kernels within TRISO compacts. Assessment of TRISO particle location confirmed and further quantified a non-uniform distribution of TRISO particles with the spatial distribution in the radial direction being roughly described as a dampened sinusoidal function. The amplitude and frequency of this non-uniform distribution increased with increasing packing fraction. Measured kernel-nearest neighbor distances indicated two regions along the radial surfaces of compacts where TRISO particles are more likely to be in intimate contact with one another. These regions were found: (1) at upper and lower faces of compacts (i.e., corners); (2) offset ∼10% of a compact's length from the axial center near the exterior surface. Within these regions, small quantities of defective TRISO surrogate particles (48% packing fraction) and defective LEUCO TRISO particles (40% packing fraction) were found. No defective particles were found within 25% packing fraction LEUCO TRISO compacts.